JUJUNCAO-Stem-Based Interfacial Solar-Driven Evaporator with Natural Two-Phase Composite Structures of Functional Partition and Inherent Ultralow Vaporization Enthalpy of Water for Stable and Efficient Steam Production

文献类型： 外文期刊

第一作者： Tan, Chenshu

作者： Tan, Chenshu;Wu, Xiaomei;Xia, Linmin;Su, Jiayun;Wu, Jianyu;Yu, Yan;Yang, Rilong;Tan, Chenshu;Xia, Linmin;Su, Jiayun;Wu, Jianyu;Yu, Yan;Yang, Rilong;Wu, Xiaomei

作者机构：

关键词： JUJUNCAO; interfacial solar-driven evaporation; water vaporization enthalpy; desalination; two-phasecomposite structures

期刊名称：ACS APPLIED MATERIALS & INTERFACES （ 影响因子：9.5； 五年影响因子：9.6 ）

ISSN： 1944-8244

年卷期： 2024 年 16 卷 3 期

页码：

收录情况： SCI

摘要： The interfacial solar-driven evaporation has been deemed as an environmentally friendly approach for freshwater generation. Nevertheless, there is still a challenge to obtain solar evaporators with efficient vapor production from low-cost and renewable biomass through a simple preparation process. Herein, the JUJUNCAO stem was selected as the substrate material, and a kind of interfacial solar-driven evaporator with natural two-phase composite structures and inherent ultralow water vaporization enthalpy was constructed by a dip-coating process. The natural two-phase composite structures were utilized as independent functional partition: the low-tortuosity and hydrophilic vascular bundles served as hierarchical channels for rapid water transportation and continuous steam escape, and the honeycomb-like parenchyma cells were considered natural heat insulators for effective thermal management. Furthermore, the JUJUNCAO stem exhibited inherent ultralow water vaporization enthalpy which was only 1.15 kJ g(-1). Benefiting from the natural two-phase composite structures of functional partition and inherent ultralow water vaporization enthalpy, the C-Js evaporator could achieve an evaporation rate of 2.77 kg m(-2) h(-1) with an efficiency of 85.6% under 1 sun illumination. Meanwhile, the C-Js exhibited a stable and ideal evaporation performance and metal ion rejection behavior in the actual brine desalination process. Owing to the cost-effective and simple pretreatment process, the C-Js evaporator has the potential for freshwater generation in undeveloped areas.

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