Presence, distribution and risk assessment of polycyclic aromatic hydrocarbons in rice-wheat continuous cropping soils close to five industrial parks of Suzhou, China

文献类型: 外文期刊

第一作者: Li, Yong

作者: Li, Yong;Ge, Jing;Cheng, Jin-jin;Yu, Xiang-yang;Li, Yong;Long, Ling;Ge, Jing;Yang, Li-xuan;Cheng, Jin-jin;Yu, Xiang-yang;Sun, Ling-xiang;Lu, Changying

作者机构:

关键词: Polycyclic aromatic hydrocarbons;Agricultural soils;Distribution;Principal component analysis;Risk assessment

期刊名称:CHEMOSPHERE ( 影响因子:7.086; 五年影响因子:6.956 )

ISSN:

年卷期:

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收录情况: SCI

摘要: Polycyclic aromatic hydrocarbons (PAHs) accumulated in agricultural soils are likely to threaten human health and ecosystem though the food chain, therefore, it is worth to pay more attention to soil contamination by PAHs. In this study, the presence, distribution and risk assessment of 16 priority PAHs in rice-wheat continuous cropping soils close to industrial parks of Suzhou were firstly investigated. The concentrations of the total PAHs ranged from 125.99 ng/g to 796.65 ng/g with an average of 352.94 ng/g. Phenanthrene (PHE), fluoranthene (FLT), benzo [a] anthracene (BaA) and pyrene (PYR) were the major PAHs in those soil samples. The highest level of PAHs was detected in the soils around Chemical plant and Steelworks, followed by Printed wire board, Electroplate Factory and Paper mill. The composition of PAHs in the soils around Chemical plant was dominated by 3-ring PAHs, however, the predominant compounds were 4, 5-ring PAHs in the soils around other four factories. Meanwhile, the concentration of the total PAHs in the soils close to the factories showed a higher level of PAHs in November (during rice harvest) than that in June (during wheat harvest). Different with other rings of PAHs, 3-ring PAHs in the soils around Chemical plant and Steelworks had a higher concentration in June. The results of principal component analysis and isomeric ratio analysis suggested that PAHs in the studied areas mainly originated from biomass, coal and petroleum combustion. The risk assessment indicated that higher carcinogenic risk was found in those sites closer to the industrial park. (C) 2017 Elsevier Ltd. All rights reserved.

分类号: X5

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