Effects of Aging Biodegradable Agricultural Films on Soil Physicochemical Properties and Heavy Metal Speciation

文献类型： 外文期刊

第一作者： Wu, Hao

作者： Wu, Hao;Peng, Tianmu;Li, Xueya;Zhao, Yang;Huang, Fengshuo;Huang, Qing;Wang, Xu;Guo, Peng;Lyu, Mingfu;Yin, Junhua;Liu, Qin;Gouda, Shaban;Mohamed, Ibrahim

作者机构：

关键词： biodegradable agricultural film; DOM; soil pH; enzyme activity; heavy metal speciation

期刊名称：TOXICS （ 影响因子：4.1； 五年影响因子：4.6 ）

ISSN：

年卷期： 2025 年 13 卷 4 期

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收录情况： SCI

摘要： Through soil incubation experiments, the effects of aged PBAT + PLA (polybutylene adipate terephthalate + polylactic acid) film fragments were analyzed. Surface characteristics and chemical structures of the films changed significantly after one (T2) and two years (T1) of aging compared to new films (T3). Both new and aged fragments reduced soil pH, altered enzyme activities, and influenced dissolved organic matter (DOM) fluorescence. Alkaline phosphatase activity declined by 33.2%, 23.8%, and 11.6% for T1, T2, and T3, respectively, while urease and sucrase activities increased in a time-dependent manner. The degree of soil humification rose by 66.4%, 60.4%, 49.3%, and 88.6% for T1, T2, T3, and T4, respectively, compared to the control (CK). Aged films exhibited stronger DOM fluorescence intensity than new films. Tessier extraction analysis revealed a decrease in exchangeable Cd by 22.9%, 13.1%, and 10.2% for T1, T2, and T3, respectively, while organically bound Cu increased. Correlation analysis indicated a significant positive relationship between soil humification and heavy metal bioavailability. These findings provide insight into the ecological effects of biodegradable agricultural films, offering a theoretical foundation for assessing their environmental risks and safety.

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