文献类型： 外文期刊
第一作者： Cai, Changyong
作者： Cai, Changyong;Gong, Huimin;Wu, Shuanggen;Liu, Song;Dong, Shengyi;Li, Fenfang;Tan, Zhijian
作者机构：
关键词： Supramolecular polymers; Supramolecular adhesives; High/low temperature resistances; Real-time monitoring; Hydrogen bonding formation
期刊名称：CHEMICAL ENGINEERING JOURNAL （ 影响因子：16.744； 五年影响因子：14.61 ）
ISSN： 1385-8947
年卷期： 2023 年 451 卷
页码：
收录情况： SCI
摘要： A supramolecular approach was applied to the construction of adhesive materials with excellent temperature resistance and strong adhesion capacity. Supramolecular hot-molten glues were prepared from two small compounds, acrylic acid (A) and choline chloride (C), using a combination of molecular recognition (formation of supramonomers) and supramolecular polymerization (formation of cross-linked polymers). The coexistence of covalent poly(A) backbones and non-covalent crosslinker C units enabled the poly(A-C)s to display tough adhesion effects with long-term stability at high (150 degrees C, 5.18 MPa) and low temperatures (-196 degrees C, 9.52 MPa) without any additives. Real-time and quantitative monitoring of the adhesion behavior of poly(A-C)s was successfully realized over a wide temperature range of -80 to 150 degrees C, using a customized device that allowed for easy monitoring of the adhesion duration, attenuation, and failure. Importantly, adhesion failure was visualized and wirelessly alarmed.
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