"Memory catalysis": Extending the photocatalytic antibacterial performance of a palladium-modified ZnO nanocomposite

文献类型: 外文期刊

第一作者: Zhang, Jingtao

作者: Zhang, Jingtao;Zhu, Mengzhen;Liu, Shurui;Zhai, Mengwan;Yao, Jing;Wang, Guanghui;Liu, Bingkun;Li, Junyang;Perego, Patrizia;Sun, Xiaodong;Liu, Shurui;Zhang, Jingtao;Liu, Bingkun

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关键词: PdO-ZnO nanocomposite; Photocatalysis; Antibacterial; Optical "memory"; Cytotoxicity test

期刊名称:JOURNAL OF WATER PROCESS ENGINEERING ( 影响因子:7.0; 五年影响因子:6.7 )

ISSN: 2214-7144

年卷期: 2023 年 54 卷

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收录情况: SCI

摘要: In this study, Pd-ZnO nanocomposite was synthesized via the facile solvothermal method. Then, PdO-ZnO was obtained by continuing calcination of the synthesized Pd-ZnO. X-ray Diffraction (XRD), Transmission Electron Microscope (TEM), and X-ray Photoelectron Spectroscopy (XPS) tests showed that Pd was converted to PdO in the process of calcination. The photocatalytic sterilization experiment showed that in the 3 % Pd-ZnO system, 2 x 107 CFU/mL of E. coli was completely killed within 3 h, while 3 % PdO-ZnO took 1.5 h. In electron spin resonance (ESR) tests on PdO-ZnO, The & BULL;OH and & BULL;O2- signals can be detected under light and within 20 min after the end of light. 1 x 105 CFU/mL of E. coli were killed within 1 h by the optical "memory" effect of PdO-ZnO. PdO-ZnO inactivates E. coli by disrupting the membrane structure of bacteria as demonstrated by scanning electron microscopy (SEM) test. PdO-ZnO is non-toxic and can be demonstrated through cytotoxicity experiments on HTT2.

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