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PCDD/Fs emissions from secondary copper production synergistically controlled by fabric filters and desulfurization

文献类型： 外文期刊

作者： Li, Haifeng 1 ; Liu, Wenbin 2 ; Lu, Anxiang 1 ; Li, Cheng 1 ; Die, Qingqi 1 ; Lei, Rongrong 2 ; Wu, Xiaolin 2 ;

作者机构： 1.Beijing Res Ctr Agr Stand & Testing, Beijing Municipal Key Lab Agr Environm Monitoring, Beijing 100097, Peoples R China

2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Beijing 100085, Peoples R China

3.UCAS, Hangzhou Inst Adv Study, Hangzhou 310024, Peoples R China

4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

关键词： PCDD/Fs; Secondary copper; Desulfurization; Fabric filter; Removal efficiency

期刊名称：ENVIRONMENTAL POLLUTION （ 影响因子：8.071； 五年影响因子：8.35 ）

ISSN： 0269-7491

年卷期： 2021 年 270 卷

页码：

收录情况： SCI

摘要： The effects of fabric filters and desulfurization systems during secondary copper smelting on polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) concentrations, emission coefficients, and profiles were studied in an oxygen-rich smelting furnace and an anode furnace. In the anode furnace, the toxic equivalent (TEQ) concentration ranges were 0.106-1.04 ng World Health Organization (WHO)-TEQ/ m(3) at the fabric filters inlet and 0.027-0.17 ng WHO-TEQ/m(3) at the outlet. For the oxygen-rich smelting furnace, the TEQ concentration ranges were 1.21-1.93 and 0.010-0.019 ng WHO-TEQ/m(3) at the desulfurization system inlet and outlet, respectively. The TEQs in the outlet stack gases of the desulfurization system from the anode furnace were 0.0041-0.016 ng WHO-TEQ/m(3). It is likely that PCDD/Fs that were taken away from the stack gases were adsorbed by the fly ash and gypsum. Solid residues were the dominant release routes for PCDD/Fs. PCDD/Fs congener and homologue profiles of stack gases from different smelting stages were similar. The contributions of more chlorinated homologues from the anode furnace decreased observably after the stack gases passed through the fabric filters. However, the desulfurization process did not greatly change the PCDD/Fs homologue profiles. Overall, both the fabric filters and desulfurization systems showed excellent removal efficiencies for PCDD/Fs in the stack gases, which reduced the TEQ emissions to well below the 0.5 ng WHO-TEQ/m(3) to achieve standard discharge. (C) 2020 Elsevier Ltd. All rights reserved.

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