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A well-organized graphene nanostructure for versatile strain-sensing application constructed by a covalently bonded graphene/rubber interface

文献类型： 外文期刊

作者： Guo, Quanquan 1 ; Luo, Yongyue 2 ; Liu, Jize 1 ; Zhang, Xinxing 1 ; Lu, Canhui 1 ;

作者机构： 1.Sichuan Univ, Polymer Res Inst, State Key Lab Polymer Mat Engn, Chengdu 610065, Sichuan, Peoples R China

2.Chinese Acad Trop Agr Sci, Agr Prod Proc Res Inst, Zhanjiang 524001, Peoples R China

期刊名称：JOURNAL OF MATERIALS CHEMISTRY C （ 影响因子：7.393； 五年影响因子：6.853 ）

ISSN： 2050-7526

年卷期： 2018 年 6 卷 8 期

页码：

收录情况： SCI

摘要： Graphene/rubber nanocomposites have attracted increasing attention for their fantastic applications in varied wearable electronics. However, the mechanical and functional properties of graphene/rubber nanocomposites are often limited by their weak interfacial interactions, such as ionic and hydrogen bonding. Here, we propose a covalently bonded graphene/rubber nanocomposite with a well-organized graphene nanostructure for versatile strain-sensing applications. Briefly, biological phytic acid was chosen as a covalent-bonding bridge to co-crosslink graphene oxide nanosheets and epoxidized natural rubber chains via the ring-opening reaction of epoxy groups. Benefiting from the covalently bonded interface, the obtained nanocomposite exhibited dramatically enhanced mechanical properties. Compared with the sulfur-cured sample, the tensile strength and elongation at break increased by 67.43% and 116.55%, respectively. Moreover, the covalent linkage facilitates the formation of a well-organized graphene network, which remarkably enhances the sensitivity and stability of the as-prepared strain sensors. The resultant sensors can monitor both large-scale and tiny human motion and exhibit great potential in the application of sign language recognition. This covalently bonded graphene/rubber interface opens the door to tailored design and low-cost fabrication of well-organized graphene nanostructures for multifunctional applications in electronic sensors, electromagnetic shielding materials, actuators for artificial muscles, etc.

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