Non-targeted profiling of aldehydes and ketones in coffee beans via isotope labelling-assisted UHPLC-Q-Orbitrap-MS and effects of roasting
文献类型: 外文期刊
作者: Chen, Han 1 ; Dong, Wenjiang 2 ; Liu, Meiyan 1 ; Li, Siyu 1 ; Wang, Gang 3 ; Ren, Dabing 1 ; Yi, Lunzhao 1 ;
作者机构: 1.Kunming Univ Sci & Technol, Fac Food Sci & Engn, Kunming 650500, Peoples R China
2.Chinese Acad Trop Agr Sci, Spice & Beverage Res Inst, Wanning 571533, Peoples R China
3.Kunming Gemmy Food Co LTD, Kunming 650101, Peoples R China
关键词: Coffee bean; Roasting degree; Isotope labelling; Aldehyde-ketone profile; LC-MS
期刊名称:JOURNAL OF FOOD COMPOSITION AND ANALYSIS ( 影响因子:4.6; 五年影响因子:4.6 )
ISSN: 0889-1575
年卷期: 2025 年 139 卷
页码:
收录情况: SCI
摘要: This study aimed to investigate the aldehydes and ketones (AKs) composition in coffee beans, particularly assess the differences between green and roasted beans. Using a novel isotope-labelling-assisted liquid chromatography- high-resolution mass spectrometry strategy, 142 potential AKs were identified in coffee beans extracts. Notably, the presence of tri-carbonyl in roasted coffee beans is revealed for the first time. Compared to green beans (GB), roasted beans showed a much higher abundance of AKs, highlighting the crucial role of roasting in the formation of these compounds. The total content indicated that unsaturated aliphatic AKs were abundant in GB, whereas other groups of AKs, such as diketones, furfurals, and tri-carbonyls, were present at higher levels in roasted beans. Roasting significantly increased the contents of 2-methylbutyraldehyde, acetoin, acetol, pyruvic acid, 5hydroxymethylfurfural, methylglyoxal, 2,3-butanedione, 2,3-pentanedione, and 2,3-hexanedione, which were 4-83 times more than those in GB. Some of them are intermediates for subsequent reactions, since their content decreased with increasing roasting degrees. Moreover, 9 AKs were selected as potential markers for distinguishing between green and roasted coffee beans and could be used to monitor the degree of roasting. Overall, this study offers valuable insights for understanding the composition and changes in AKs during coffee roasting.
- 相关文献
作者其他论文 更多>>
-
Sulfury/roasty fading indicators in roasted coffees: Their contribution and applicability in coffee freshness perception and prediction
作者:Zhou, Xiong;Gu, Yin;Ren, Dabing;Li, Siyu;Yi, Lunzhao;Zhou, Xiong;Yu, Xinxin;Dong, Wenjiang;Dong, Wenjiang;Diao, Yuhua;Zhang, Jiawen;Wang, Gang
关键词:Coffee; Accelerated storage; Sulfury/roasty aroma; Volatile compounds; Shelf life prediction model
-
Exploration of interaction mechanisms and functional properties of coffee flavonoids and β-casein via multispectroscopy and molecular dynamics simulation
作者:Zhang, Jiyue;Zhai, Xiaoyu;Yu, Xinxin;Hu, Rongsuo;Dong, Wenjiang;Zhang, Jiyue;Yu, Xinxin;Qiu, Minghua;Zhai, Xiaoyu;Dong, Wenjiang
关键词:Coffee flavonoids; beta-Casein; Interaction mechanism; Multispectroscopy; Molecular docking
-
Optimization process of coffee pulp wines combined with the artificial neural network and response surface methodology
作者:Hu, Rongsuo;Zhao, Liyan;Hu, Rongsuo;Xu, Fei;Dong, Wenjiang;Hu, Rongsuo;Xu, Fei;Dong, Wenjiang;Zhao, Liyan
关键词:Coffee pulp wine; Process optimization; RSM; ANN-GA
-
Effect of three pectin fractions from muskmelon on the formation of volatile sulfur compounds produced from methionine-sugars Maillard reaction
作者:Pan, Xin;Bi, Shuang;Xu, Yingying;Cai, Yanpei;Lao, Fei;Wu, Jihong;Bi, Shuang;Ai, Jingya;Dong, Wenjiang
关键词:Muskmelon pectin; Volatile sulfur compounds; Maillard reaction; Pathway; Dicarbonyl compounds
-
The impact of extraction methods on the structural and physicochemical properties of polysaccharides from spent coffee grounds and their potential as food packaging co-ingredients
作者:Han, Qiuyu;Zhang, Suyun;Zhang, Yue;Fan, Xinlong;Li, Wei;Dong, Wenjiang;Wang, Xiaohui;Zhang, Yue
关键词:Spent coffee grounds; Polysaccharide extraction; Emulsification; Composite film; Spent coffee grounds; Polysaccharide extraction; Emulsification; Composite film
-
Evaluation of the effects of Saccharomyces cerevisiae fermentation on the non-volatile compounds in semi-dry coffee beans using widely targeted metabolomics analysis
作者:Yu, Xinxin;Huang, Mei;Hu, Rongsuo;Dong, Wenjiang;Fu, Xingfei;Huang, Mei
关键词:Coffee; Non-volatile compounds; Saccharomyces cerevisiae; Widely targeted metabolomics
-
The composition and bioactivity of bound polyphenols from coffee dietary fiber during in vitro Simulating digestion
作者:Yu, Xinxin;Zhang, Jiyue;Long, Yuzhou;Dong, Wenjiang;Shao, Fangfang;Yu, Xinxin;Zhang, Jiyue;Long, Yuzhou;Dong, Wenjiang
关键词:Coffee peel soluble dietary fiber; Bound polyphenols; UPLC-MS/MS; Simulating digestion



