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Elastic, super-hydrophobic and biodegradable chitosan sponges fabricated for oil/water separation

文献类型： 外文期刊

作者： Liang, Fengyan 1 ; Hou, Tingting 1 ; Li, Sidong 1 ; Liao, Lusheng 2 ; Li, Puwang 3 ; Li, Chengpeng 1 ;

作者机构： 1.Guangdong Ocean Univ, Sch Chem & Environm Sci, Zhanjiang 524088, Peoples R China

2.Chinese Acad Trop Agr Sci, Guangdong Prov Key Lab Nat Rubber Proc, Agr Prod Proc Res Inst, Zhanjiang 524001, Peoples R China

3.Chinese Acad Trop Agr Sci, Agr Prod Proc Res Inst, Zhanjiang 524001, Peoples R China

关键词： Chitosan; Elasticity; Super-hydrophobicity; Biodegradability; Oil/water separation

期刊名称：JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING （ 影响因子：5.909； 五年影响因子：5.649 ）

ISSN：

年卷期： 2021 年 9 卷 5 期

页码：

收录情况： SCI

摘要： Due to easy availability and biodegradability, chitosan (CS)-based porous adsorbents have attracted significant interest in oil-spill and organic solvent removal. Herein, a multi-network CS-based sponge was fabricated via ion and hydrogen bond cross-linking using lemon, followed by covalent cross-linking via heptanal, in-situ loading of Fe3O4-polydopamine (PDA) particles and polylactic acid (PLA) coating. The as-fabricated sponge was system-atically characterized by Fourier transform-infrared spectrometry (FT-IR), X-ray diffraction (XRD), vibrating sample magnetometer (VSM), X-ray photoelectron spectroscopy (XPS), scanning electron microscope (SEM), transmission electron microscope (TEM), static water contact angles (WCA) and so on. The as-fabricated CS-based sponge exhibits excellent elasticity, which could be compressed to large strains (80%) at a relatively high stress (0.685 MPa). The WCA of the targeted sponge can reach to 152.2 +/- 1.2o after multiple surface func-tionalization. In addition, the degradation rate of the as-fabricated sponge can still reach 45.01 +/- 1.11% within 15 days. Particularly, the sponge could selectively adsorb oil/organic solvent with up to 50 times of its own weight, and effectively separate the surfactant-stabilized oil-in-water emulsion with a flux of 8753 +/- 423.56 L m(-2) h(-1). Last but not least, the sponge can be driven and recycled magnetically. In conclusion, this promising multifunctional sponge can be applied as a new absorbent for oil-water separation.

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