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The influence of using different types of modified vermiculite cover on ammonia mitigation from animal slurry storage: The role of sulfuric acid

文献类型： 外文期刊

作者： Wang, Yue 1 ; Wang, Shunli 1 ; Ni, Ji-Qin 3 ; Shi, Shengwei 4 ; Su, Xiaoli 5 ; Zhang, Jingyu 4 ; Zhu, Zhiping 1 ; Dong, Hongmin 1 ;

作者机构： 1.Chinese Acad Agr Sci, Inst Environm & Sustainable Dev Agr, Beijing 100081, Peoples R China

2.Beijing Acad Agr & Forestry Sci, Inst Plant Nutr & Resources, Beijing 100087, Peoples R China

3.Purdue Univ, Dept Agr & Biol Engn, W Lafayette, IN 47907 USA

4.Beijing Univ Agr, Coll Biosci & Resources Environm, Beijing 100083, Peoples R China

5.Jingdezhen Ceram Univ, Coll Mat Sci & Engn, Jingdezhen 333000, Peoples R China

关键词： Nitrous oxide; Adsorption; Acidification; Coverage; Nitrification

期刊名称：WASTE MANAGEMENT （ 影响因子：8.1； 五年影响因子：8.7 ）

ISSN： 0956-053X

年卷期： 2024 年 178 卷

页码：

收录情况： SCI

摘要： Animal slurry storage is an important ammonia (NH3) emission source. Sulfuric acid (H2SO4)-modified vermiculite coverage is a new promising technology for controlling NH3 emission from slurry storage. However, the underlying mechanisms in controlling the mitigation effect remain unclear. Here, a series of experiments to determine the effect of H2SO4 on the modified vermiculite properties, floating persistence, and NH3 mitigation effect was conducted. Results showed that abundant H2SO4 and sulfate remained on the outer surface and in the extended inner pores of the vermiculite with acidifying H+ concentrations higher than 5 M. An initial strong instantaneous acidification of surface slurry released rich carbon dioxide bubbles, strengthening cover floating performance. An acidification in the vermiculite cover layer and a good coverage inhibition interacted, being the two leading mechanisms for mitigating NH3 during initial 40-50 days of storage. The bacterial-amoA gene dominated the conversion of NH3 to nitrous oxide after 50 days of storage. Vermiculite with 5 M H+ modification reduced the NH3 emissions by 90 % within the first month of slurry storage and achieved a 64 % mitigation efficiency throughout the 84 days period. With the development of the aerial spraying equipment such as agricultural drones, acidifying vermiculite coverage hold promise as an effective method for reducing NH3 emission while absorbing nutrients from liquid slurry storage tank or lagoon. This design should now be tested under field conditions.

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