Microplastics mulch film affects the environmental behavior of adsorption and degradation of pesticide residues in soil

文献类型： 外文期刊

第一作者： Wu, Changcai

作者： Wu, Changcai;Pan, Shaodong;Shan, Yongpan;Ma, Yajie;Wang, Dan;Song, Xianpeng;Hu, Hongyan;Ren, Xiangliang;Ma, Xiaoyan;Cui, Jinjie;Ma, Yan;Wu, Changcai;Cui, Jinjie

作者机构：

关键词： Plastic mulch film; Microplastics; Pesticide; Adsorption; Degradation

期刊名称：ENVIRONMENTAL RESEARCH （ 影响因子：8.431； 五年影响因子：8.399 ）

ISSN： 0013-9351

年卷期： 2022 年 214 卷

页码：

收录情况： SCI

摘要： Plastic pollution in the soil ecosystem is currently receiving worldwide attention. However, little is known whether the presence of microplastics (MPs) in soil will affect the environmental behavior of pesticide residues in soil. Here, the effect of the addition of new mulch MPs (New-MPs), aged mulch MPs (Aged-MPs) and biodegradable mulch MPs (BioD-MPs) on the adsorption and degradation behaviors of two pesticides (imidacloprid and flumioxazin) in soil was investigated. Three MPs slowed down rapid adsorption stage of pesticides in soil and delayed the time to reach adsorption equilibrium. Adsorption rates: Soil > Soil + New-MPs > Soil + Aged-MPs > Soil + BioD-MPs. Three MPs enhanced the adsorption strength of the soil system for the two pesticides, and the aging treatment of the MPs enhanced this effect. Three MPs affected the degradation process of the two pesticides. New-MPs promoted the degradation of two pesticides imidacloprid and flumioxazin, and the degradation half-lives were shortened to 0.93 and 0.85 times, respectively; while Aged-Mps and BioD-MPs delayed the degradation process of two pesticides, and the degradation half-lives were extended to 1.64 times and 1.21 times, respectively. The effect was more significant with the increase of MPs and pesticides concentration. Pesticide polarity, surface structure and functional groups of MPs are potentially important reasons for the differences in adsorption and degradation of MPs-soil systems. Our findings provide a deep insight into understanding the mechanism of interaction between MPs and pesticide residues in soil environment.

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