Preliminary investigation of phosphorus adsorption onto two types of iron oxide-organic matter complexes

文献类型： 外文期刊

第一作者： Yan, Jinlong

作者： Yan, Jinlong;Jiang, Tao;Lu, Song;Wang, Qilei;Wei, Shiqiang;Jiang, Tao;Yao, Ying

作者机构：

关键词： Phosphorus;Ferrihydrite-humic acid complex;Goethite-humic acid complex;Adsorption

期刊名称：JOURNAL OF ENVIRONMENTAL SCIENCES （ 影响因子：5.9； 五年影响因子：5.6 ）

ISSN：

年卷期：

页码：

收录情况： SCI

摘要： Iron oxide (FeO) coated by natural organic matter (NOM) is ubiquitous. The associations of minerals with organic matter (OM) significantly changes their surface properties and reactivity, and thus affect the environmental fate of pollutants, including nutrients (e.g., phosphorus (P)). In this study, ferrihydrite/goethite-humic acid (FH/GE-HA) complexes were prepared and their adsorption characteristics on P at various pH and ionic strength were investigated. The results indicated that the FeO-OM complexes showed a decreased P adsorption capacity in comparison with bare FeO. The maximum adsorption capacity (Q(max)) decreased in the order of FH (22.17 mg/g) > FH-HA (5.43 mg/g) > GE (4.67 mg/g) > GE-HA (3.27 mg/g). After coating with HA, the amorphous FH-HA complex still showed higher P adsorption than the crystalline GE-HA complex. The decreased P adsorption observed might be attributed to changes of the FeO surface charges caused by OM association. The dependence of P adsorption on the specific surface area of adsorbents suggests that the FeO component in the complexes is still the main contributor for the adsorption surfaces. The P adsorptions on FeO-HA complexes decreased with increasing initial pH or decreasing initial ionic strength. A strong dependence of P adsorption on ionic strength and pH may demonstrate that outer-sphere complexes between the OM component on the surface and P possibly coexist with inner-sphere surface complexes between the FeO component and P. Therefore, previous over-emphasis on the contributions of original minerals to P immobilization possibly over-estimates the P loading capacity of soils, especially in humic-rich areas. (C) 2015 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

分类号： X5

  • 相关文献

[1]Water hyacinth (Eichhornia crassipes) waste as an adsorbent for phosphorus removal from swine wastewater. Chen, Xi,Chen, Xiuxia,Wan, Xianwei,Huang, Qin,Weng, Boqi.

[2]Identification of quantitative trait locus of zinc and phosphorus density in wheat (Triticum aestivum L.) grain. Shi, Rongli,Zhang, Fusuo,Zou, Chunqin,Li, Hongwei,Tong, Yiping,Jing, Ruilian.

[3]Changes in the soil environment from excessive application of fertilizers and manures to two contrasting intensive cropping systems on the North China Plain. Ju, X. T.,Kou, C. L.,Christie, P.,Dou, Z. X.,Zhang, F. S..

[4]Adsorption and photocatalytic degradation of phenol over TiO2/ACF. Fan, CM,Min, YQ,Hao, XG,Sun, YP,Li, XJ,Li, FB. 2003

[5]Study on the Effect of Carboxyl Bagasse Hemicellulose on Heavy Metal Adsorption. Liu, Xinliang,Zhu, Hongxiang,Li, Zhoujun,Lu, Yiguan,Wu, Fusheng,Wang, Shuangfei,Weng, Mengling. 2012

[6]Photocatalytic reaction kinetics model based on electrical double layer theory - II. Surface complexation model of methyl orange adsorption on TiO2 surface. Li, XJ,Li, FB,Gu, GB,Liu, S,Wang, LY,Liang, YY. 2003

[7]Simulation of adsorption of gold nanoparticles carried by gas ascending from the Earth's interior in alluvial cover of the middle-lower reaches of the Yangtze River. Cao, J. J.,Hu, X. Y.,Jiang, Z. T.,Li, H. W.,Zou, X. Z.. 2010

[8]Adsorption of Cu(II) on humic acids derived from different organic materials. Ji Fan,Zhang Jin-jing,Gao Qiang,Wu Jing-gui,Zhao Lan-po,Wang Shuai,Wang Li-chun,Zheng Li-rong. 2015

[9]Preparation of Tetraethylenepentamine Modified Magnetic Graphene Oxide for Adsorption of Dyes from Aqueous Solution. Tang, Xiaosheng,Tang, Xiaosheng,Tang, Xiaosheng,Tang, Ping,Liu, Liangliang,Tang, Ping. 2018

[10]Adsorption and photocatalytic decomposition of roxarsone by TiO2 and its mechanism. Lu, Donglei,Wang, Wei,Yuan, Shoujun,Hu, Zhen-Hu,Ji, Feng,Wang, Wei,Yuan, Shoujun,Hu, Zhen-Hu,Chen, Tianhu. 2014

[11]Study on the tolerance and adsorption of five heavy metal ions by a radiation-resistant Acinetobacter sp.. Zhu Jing,Xie Yu-Qing,Song Su-Qin,Zhang Zhi-Dong,Wang Wei,Gu Mei-Ying,Tang Qi-Yong. 2013

[12]Effects of Biochar Amendment on Chloropicrin Adsorption and Degradation in Soil. Wang, Qiuxia,Yan, Dongdong,Fang, Wensheng,Mao, Liangang,Li, Yuan,Ouyang, Canbin,Guo, Meixia,Cao, Aocheng,Wang, Dong. 2016

[13]Removal of roxarsone from aqueous solution by Fe/La-modified montmorillonite. Wang, Ya-Jiao,Wang, Wei,Yuan, Shou-Jun,Hu, Zhen-Hu,Ji, Feng,Wang, Wei,Yuan, Shou-Jun,Hu, Zhen-Hu. 2016

[14]Phosphorus Adsorption and Bioavailability in a Paddy Soil Amended with Pig Manure Compost and Decaying Rice Straw. Liang, Yongchao,Guo, Bin,Liang, Yongchao,Li, Zhaojun,Han, Fengxiang. 2009

[15]The Effect of Two Types of Biochars on the Efficacy, Emission, Degradation, and Adsorption of the Fumigant Methyl Isothiocyanate. Cao, Aocheng,Yan, Dongdong,Han, Dawei,Huang, Bin,Li, Jun,Liu, Xiaoman,Guo, Meixia,Wang, Qiuxia. 2017

[16]XPS and SEM Spectroscopy Study of Hyperdispersant on Atrazine Surface. Xu Yan,Ma Chao,Zhang Ping,Cai Meng-ling,Wu Xue-min,Sun Bao-li. 2011

[17]Adsorption characteristics of 4-hydroxy-3-aminophenylarsonic acid (HAPA) onto anaerobic granular sludge. Li, Jun-Chao,Yuan, Shou-Jun,Wang, Wei,Hu, Zhen-Hu,Ji, Feng,Yuan, Shou-Jun,Wang, Wei,Hu, Zhen-Hu. 2016

[18]Preparation of porous carbon directly from hydrothermal carbonization of fructose and phloroglucinol for adsorption of tetracycline. Bai, Chen-Xi,Bai, Chen-Xi,Shen, Feng,Qi, Xin-Hua. 2017

[19]Adsorption of Chloride Anion from Aqueous Solution by Calcined (Mg-Al) Hydrotalcites of Different Mg/Al Ratio. Wan, Dongjin,Liu, Yongde,Lu, Ting,Qu, Dan,Xiao, Hua,Xu, Wenqing. 2011

[20]Removal of Cd, Pb and Cu from Water Using Thiol and Humic Acid Functionalized Fe2O3 Nanoparticles. Wang Meng,Chen Shibao. 2012

作者其他论文 更多>>

微信小程序