Underestimation of phosphorus fraction change in the supernatant after phosphorus adsorption onto iron oxides and iron oxide-natural organic matter complexes

文献类型： 外文期刊

第一作者： Yan, Jinlong

作者： Yan, Jinlong;Wang, Jun;Wei, Shiqiang;Jiang, Tao;Yao, Ying;Cai, Yuanli;Green, Nelson W.

作者机构：

关键词： Phosphorus;Fraction;Ultrafiltration;Natural organic matter;Iron-DOM;Iron oxide-humic acid complexes

期刊名称：JOURNAL OF ENVIRONMENTAL SCIENCES （ 影响因子：5.9； 五年影响因子：5.6 ）

ISSN：

年卷期：

页码：

收录情况： SCI

摘要： The phosphorus (P) fraction distribution and formation mechanism in the supematant after P adsorption onto iron oxides and iron oxide-humic acid (HA) complexes were analyzed using the ultrafiltration method in this study. With an initial P concentration of 20 mg/L (I = 0.01 mol/L and pH = 7), it was shown that the colloid (1 kDa-0.45 gm) component of P accounted for 10.6%, 11.6%, 6.5%, and 4.0% of remaining total P concentration in the supematant after P adsorption onto ferrihydrite (FH), goethite (GE), ferrihydrite-humic acid complex (FH-HA), goethite-humic acid complex (GE-HA), respectively. The <1 kDa component of P was still the predominant fraction in the supematant, and underestimated colloidal P accounted for 2.2%, 55.1%, 45.5%, and 38.7% of P adsorption onto the solid surface of FH, FH-HA, GE and GE-HA, respectively. Thus, the colloid P could not be neglected. Notably, it could be interpreted that Fe3+ hydrolysis from the adsorbents followed by the formation of colloidal hydrous ferric oxide aggregates was the main mechanism for the formation of the colloid P in the supematant. And colloidal adsorbent particles co-existing in the supernatant were another important reason for it. Additionally, dissolve organic matter dissolved from iron oxide-HA complexes could occupy large adsorption sites of colloidal iron causing less colloid P in the supematant. Ultimately, we believe that the findings can provide a new way to deeply interpret the geochemical cycling of P, even when considering other contaminants such as organic pollutants, heavy metal ions, and arsenate at the sediment/soil-water interface in the real environment. (C) 2016 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.

分类号： X5

  • 相关文献

[1]Production of concentrated kiwifruit juice by integrated membrane process. Cassano, A,Jiao, B,Drioli, E.

[2]Fraction characteristics of rare earth elements in the surface sediment of Bohai Bay, North China. Xu, Yayan,Song, Jinming,Duan, Liqin,Li, Xuegang,Yuan, Huamao,Li, Ning,Zhang, Peng,Zhang, Ying,Xu, Sisi,Zhang, Mo,Wu, Xiaodan,Yin, Xuebo,Xu, Yayan,Xu, Yayan,Duan, Liqin,Zhang, Peng,Zhang, Ying,Xu, Sisi,Zhang, Mo,Wu, Xiaodan.

[3]Composition of dissolved organic matter (DOM) from periodically submerged soils in the Three Gorges Reservoir areas as determined by elemental and optical analysis, infrared spectroscopy, pyrolysis-GC-MS and thermally assisted hydrolysis and methylation. Jiang, Tao,Liang, Jian,Wei, Shiqiang,Wang, Dingyong,Jiang, Tao,Kaal, Joeri,Kaal, Joeri,Zhang, Yaoling,Green, Nelson W.. 2017

[4]Effect of Abiotic Factors on the Mercury Reduction Process by Humic Acids in Aqueous Systems. Jiang Tao,Wei Shi-Qiang,Li Meng-Jie,Li Xue-Mei,Wang Qiang,Luo Chang,Jiang Tao,Wei Shi-Qiang,Wang Qiang,Flanagan, D. C..

[5]Identification of quantitative trait locus of zinc and phosphorus density in wheat (Triticum aestivum L.) grain. Shi, Rongli,Zhang, Fusuo,Zou, Chunqin,Li, Hongwei,Tong, Yiping,Jing, Ruilian.

[6]Changes in the soil environment from excessive application of fertilizers and manures to two contrasting intensive cropping systems on the North China Plain. Ju, X. T.,Kou, C. L.,Christie, P.,Dou, Z. X.,Zhang, F. S..

[7]Analysis of Xanthine Oxidase Inhibitors from Puerariae flos Using Centrifugal Ultrafiltration Coupled with HPLC-MS. Liangliang Liu,Li, Defang,Aiping Xiao,Lei Ma,Defang Li. 2017

[8]Effects of wheat gluten hydrolysates fractionated by different methods on the growth and fermentation performances of brewer's yeast under high gravity fermentation. Zhou, Yongjing,Yang, Huirong,Cui, Chun,Zhao, Haifeng,Zong, Xuyan,Mu, Lixia. 2018

[9]Isolation of -Amylase Inhibitors from Kadsura longipedunculata Using a High-Speed Counter-Current Chromatography Target Guided by Centrifugal Ultrafiltration with LC-MS. Cen, Yin,Chen, Xiaoqing,Xiao, Aiping,Liu, Liangliang.

[10]Separation and properties of polysaccharides from asparagus (Officinalis L) old stalks. Song, Jia,Qian, Haifeng,Ma, Yue,Zhang, Chao,Zhao, Xiaoyan. 2012

[11]Fouling of extracellular algal organic matter during ultrafiltration: The influence of iron and the fouling mechanism. Huang, Weiwei,Zhou, Wenzong,Lv, Weiguang,Huang, Weiwei,Hu, Mengliu,Qin, Xiao,Dong, Bingzhi. 2017

[12]Effects of combined ozone and PAC pretreatment on ultrafiltration membrane fouling control and mechanisms. Huang, Weiwei,Zhou, Wenzong,Lv, Weiguang,Hu, Mengliu,Chu, Huaqiang,Dong, Bingzhi,Wang, Lin.

[13]Some characteristics and functional properties of rapeseed protein prepared by ultrasonication, ultrafiltration and isoelectric precipitation. Dong, Xu-Yan,Zhao, Yuan-Di,Dong, Xu-Yan,Guo, Lu-Lu,Wei, Fang,Li, Ju-Fang,Jiang, Mu-Lan,Li, Guang-Ming,Chen, Hong. 2011

[14]Separation of antihypertensive peptides derived from soybean protein isolated with ultrafiltration technology. Hu, Shaoxin,Jiang, Lianzhou,Li, Yang,Sui, Xiaonan,Pan, Yuanyuan. 2012

[15]Effects of thermal, microwave, and ultrasound pretreatments on antioxidative capacity of enzymatic milk protein concentrate hydrolysates. Uluko, Hankie,Zhang, Shuwen,Liu, Lu,Tsakama, Madalitso,Lu, Jing,Lv, Jiaping,Uluko, Hankie,Tsakama, Madalitso.

[16]Long-term pig manure application reduces the requirement of chemical phosphorus and potassium in two rice-wheat sites in subtropical China. Xu, M.,He, X.,He, X.,He, X.,He, X.,Li, S.,Sun, X.. 2011

[17]Estimation the leaf phosphorus concentration of litchi (Litchi chinensis Sonn.) at different growth stages by canopy reflectance. Wang, Chongyang,Chen, Shuisen,Li, Dan,Liu, Wei,Huang, Siyu,Peng, Zhiping. 2015

[18]Nitrogen use efficiency in a wheat-corn cropping system from 15 years of manure and fertilizer applications. Duan, Yinghua,Xu, Minggang,Liu, Hongbin,Wang, Bairen,Gao, Suduan,Yang, Xueyun,Huang, Shaomin. 2014

[19]Fishmeal can be totally replaced by plant protein blend at two protein levels in diets of juvenile Siberian sturgeon, Acipenser baerii Brandt. Yun, B.,Xue, M.,Wang, J.,Sheng, H.,Zheng, Y.,Wu, X.,Li, J.,Yun, B.,Xue, M.. 2014

[20]Efficiency, economics, and environmental implications of phosphorus resource use and the fertilizer industry in China. Oenema, Oene,Zhang, Weifeng,Fan, Mingsheng,Zhang, Fusuo,Ma, Wenqi,Ji, Yuexiu. 2008

作者其他论文 更多>>

微信小程序