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The effect of COVID-19 epidemic and sandstorm on distribution of short-, medium-, and long-chain chlorinated paraffins in outdoor atmosphere of Xi'an, Northwest China

文献类型： 外文期刊

作者： Liu, Xiuqun 1 ; Huang, Xiaomei 2 ; Song, Han 3 ; Wang, Jingzhi 1 ; Li, Jiayu 5 ; Li, Xi 1 ; Dong, Zhibao 1 ; Xing, Li 1 ; Cao, Junji 5 ;

作者机构： 1.Shaanxi Normal Univ, Natl Demonstrat Ctr Expt Geog Educ, Sch Geog & Tourism, Xian, Peoples R China

2.Guangdong Acad Agr Sci, Inst Qual Stand & Monitoring Technol Agroprod, Guangzhou, Peoples R China

3.Henan Acad Sci, High & New Technol Res Ctr, Hongzhuan Rd, Zhengzhou, Peoples R China

4.Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, State Key Lab Loess & Quaternary Geol SKLLQG, Xian, Peoples R China

5.Univ Miami, Mech & Aerosp Engn, Coral Gables, FL USA

6.Univ Miami, Ctr Aerosol Sci & Technol, Coral Gables, FL USA

7.Chinese Acad Sci, Inst Atmospher Phys, Beijing, Peoples R China

关键词： Chlorinated paraffins; Homologue patterns; Gas-particle partitioning; Sandstorm; COVID-19 epidemic; Human exposure risks

期刊名称：ATMOSPHERIC ENVIRONMENT （ 影响因子：3.7； 五年影响因子：4.2 ）

ISSN： 1352-2310

年卷期： 2024 年 338 卷

页码：

收录情况： SCI

摘要： The short-, medium- and long-chain chlorinated paraffins (SCCPs, MCCPs, and LCCPs) were measured in outdoor fine particulate matter (PM2.5) and gas-phases in Xi'an in spring, autumn and winter of 2021, which containing two special events during this time, the sandstorms happened in spring and the COVID-19 epidemic in winter. The CPs concentrations in PM2.5 were seasonal variated, with spring (mean: 17.5 ng/m(3)) > autumn (mean: 8.6 ng/m(3)) > winter (mean: 5.8 ng/m(3)). The CPs concentrations in gas phases (mean:12.6 ng/m(3)) were lower than in PM2.5 in spring, and it showed shorter carbon chain and lower chlorinated CPs dominated in SCCPs in gas phase (C-10, C-l5,C-6) compared with in PM2.5 (C-11, Cl-6,Cl-7). The absorption was the main mechanism for the partitioning of CP in particle and gaseous phase. The shorter carbon chain CPs (C-10,C-11, C-14) with lower chlorinated (Cl-6,Cl-7) CPs dominated in SCCPs and MCCPs, while the longer carbon chain (C-25 or C-29) with Cl-6,Cl-12 dominated in the LCCPs. So, more researches about the LCCPs should be concerned. Additionally, the CPs concentrations of all samples during the sandstorms in spring were increased 30.4%-136.5% and the proportion of SCCPs was obviously elevated. CPs concentrations obviously decreased during the COVID-19 epidemic in winter, while SCCPs, MCCPs attributed comparable in autumn and winter. Potential source analysis showed that during the sandstorms in spring, atmospheric pollutants were mainly transported over a long distance from northern and northeast of Shaanxi Province, while it was mainly from local emission during the COVID-19 epidemic in winter. The health risk assessment of CPs displayed that there had no or very low inhalation exposure risks of CPs for all age groups, but the younger age groups (younger than 6 years old) should be played more attention for their not fully development of their immune and respiratory systems.

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