Enhanced Photocatalytic Activity for CO2 Reduction over a CsPbBr3/CoAl-LDH Composite: Insight into the S-Scheme Charge Transfer Mechanism
文献类型： 外文期刊
作者： Li, Deben 1 ; Zhou, Jiaxin 2 ; Zhang, Zhijie 1 ; Jiang, Ying 1 ; Dong, Zhongliang 1 ; Xu, Jiayue 1 ; Yao, Chunxia 2 ;
作者机构： 1.Shanghai Inst Technol, Sch Mat Sci & Engn, Shanghai 201418, Peoples R China
2.Shanghai Acad Agr Sci, Inst Agrofood Stand & Testing Technol, Shanghai 201403, Peoples R China
关键词： S-scheme heterojunction; CsPbBr3; photocatalysis; CO2 reduction; charge separation
期刊名称：ACS APPLIED ENERGY MATERIALS （ 影响因子：6.959； 五年影响因子：7.01 ）
ISSN： 2574-0962
年卷期：
页码：
收录情况： SCI
摘要： The construction of an S-scheme heterojunction is recognized as a promising approach to developing efficient photocatalytic systems. Herein, a novel S-scheme heterojunction of CsPbBr3 nanocrystals/CoAl layered double hydroxide (LDH) nanosheets was fabricated and applied for photocatalytic conversion of CO2. CsPbBr3/CoAl-LDH composites exhibited superior activity for CO2 photoreduction under visible light. The composite containing 60 wt % CsPbBr3 displayed the optimal photocatalytic perform-ance, which was enhanced by 2.6 and 9.9 times compared to CsPbBr3 and CoAl-LDH, respectively. Moreover, this composite also showed stable photocatalytic activity with no detectable decrease after four cycles. The formation of an S-scheme heterojunction can promote the electron-hole separation and provide a higher redox potential of the composite, thus leading to the remarkable photocatalytic performance toward CO2 reduction. This study provides a new perspective for designing and manufacturing perovskite-based S-scheme photocatalytic systems for CO2 reduction.
- 相关文献
作者其他论文 更多>>
-
Boosted antibiotic elimination over 2D/2D mesoporous CeO2/BiOCl S-scheme photocatalyst
作者：Tang, Huiling;Wang, Xuesheng;Zhang, Zhijie;Hengchao, E.;Zhou, Jiaxin;Song, Wei
关键词：S-scheme heterojunction; CeO2; BiOCl; Photocatalyst; Antibiotics
-
A novel, low-cost, and efficient separation strategy based on S-doped C3N4 for the analysis of PCDD/Fs and dioxin-like PCBs
作者：Luo, Yanli;Luo, Yanli;Liu, Chengbin;Wang, Xianli;Zhang, Qicai;Yao, Chunxia;Huang, Di;Liu, Xing;Lu, Yangyang;Song, Wei;Chen, Shanshan;Zhou, Jiaxin;Rao, Qinxiong;Song, Weiguo;Liu, Chengbin;Wang, Xianli;Zhang, Qicai;Yao, Chunxia;Huang, Di;Liu, Xing;Lu, Yangyang;Song, Wei;Chen, Shanshan;Zhou, Jiaxin;Rao, Qinxiong;Liu, Chengbin;Wang, Xianli;Zhang, Qicai;Yao, Chunxia;Huang, Di;Liu, Xing;Lu, Yangyang;Song, Wei;Chen, Shanshan;Zhou, Jiaxin;Rao, Qinxiong
关键词：PCDD/Fs; Dl-PCBs; Carbon nitride; Separation; Analysis
-
2D/2D Ni-MOF/BiOCl S-scheme heterojunction with boosted charge transfer and photocatalytic degradation of tetracycline
作者：Zhou, Jiaxin;Yao, Chunxia;Song, Weiguo;Liu, Chengbin;Song, Wei;Tang, Huiling;Zhang, Zhijie
关键词：S-scheme heterojunction; Ni-MOF; BiOCl; Photocatalyst; Tetracycline
-
0D/3D heterostructure of perovskite Cs2CuBr4 quantum dots/Bi2O3 microflower as a step-scheme photocatalyst for enhanced CO2 reduction
作者：Tang, Huiling;Wang, Xuesheng;Zhang, Zhijie;Yao, Chunxia
关键词：Step-scheme photocatalyst; Cs2CuBr4; CO2 reduction; Charge transfer
-
Occurrence and Risk Assessment of Pesticides, Phthalates, and Heavy Metal Residues in Vegetables from Hydroponic and Conventional Cultivation
作者：Chen, Shanshan;Yao, Chunxia;Zhou, Jiaxin;Song, Weiguo;Ma, Haiyao;Jin, Jing;Kai, Zhenpeng
关键词：risk assessment; hydroponic; vegetable; pesticide residues; phthalates; heavy metals
-
Cs2 CuBr4 perovskite quantum dots confined in mesoporous CuO framework as a p-n type S-scheme heterojunction for efficient CO2 photoconversion
作者：Zhang, Zhijie;Li, Xun;Tang, Huiling;Tang, Huiling;Yao, Chunxia;Wu, Junhao;Li, Kui
关键词：Photocatalytic CO 2 conversion; Mesoporous CuO; Cs 2 CuBr 4; Perovskite quantum dots; S -scheme heterojunction
-
Gradual effects of gradient concentrations of perfluorooctane sulfonate on the antioxidant ability and gut microbiota of red claw crayfish ( Cherax quadricarinatus )
作者：Hong, Shuang;Song, Weiguo;Liu, Chengbin;Yao, Chunxia;Zhu, Chenxi;Han, Mingming;Jiang, Qichen;Lv, Weiwei;Jiang, Qichen;Hong, Shuang
关键词：Gut microbes; PFOS; Antioxidant response; Cherax quadricarinatus
