Indirect photodegradation of sulfadiazine in the presence of DOM: Effects of DOM components and main seawater constituents
文献类型： 外文期刊
作者： Bai, Ying 1 ; Zhou, Yanlei 3 ; Che, Xiaowei 4 ; Li, Conghe 4 ; Cui, Zhengguo 1 ; Su, Rongguo 4 ; Qu, Keming 1 ;
作者机构： 1.Chinese Acad Fishery Sci, Yellow Sea Fisheries Res Inst, Key Lab Sustainable Dev Marine Fisheries, Minist Agr & Rural Affairs, Qingdao 266071, Peoples R China
2.Pilot Natl Lab Marine Sci & Technol Qingdao, Lab Marine Fisheries Sci & Food Prod Proc, Qingdao 266071, Peoples R China
3.Jimo Comprehens Inspect & Testing Ctr, Qingdao 266200, Peoples R China
4.Ocean Univ China, Lab Marine Chem Theory & Technol, Minist Educ, Qingdao 266100, Peoples R China
关键词： Sulfadiazine; Dissolved organic matter; Indirect photodegradation; Reactive intermediate; Fluorescence components
期刊名称：ENVIRONMENTAL POLLUTION （ 影响因子：8.071； 五年影响因子：8.35 ）
ISSN： 0269-7491
年卷期： 2021 年 268 卷
页码：
收录情况： SCI
摘要： The presence of pharmaceuticals and personal care products in coastal waters has caused concern over the past decade. Sulfadiazine (SD) is a very common antibiotic widely used as human and fishery medicine, and dissolved organic matter (DOM) plays a significant role in the indirect photodegradation of SD; however, the influence of DOM compositions on SD indirect photodegradation is poorly understood. The roles of reactive intermediates (RIs) in the indirect photolysis of SD were assessed in this study. The reactive triplet states of DOM (3DOM*) played a major role, whereas HO center dot and O-1(2) played insignificant roles. DOM was divided into four components using excitation-emission matrix spectroscopy combined with parallel factor analysis. The components included three allochthonous humic-like components and one autochthonous humic-like component. The allochthonous humic-like components contributed more to RIs generation and SD indirect photolysis than the autochthonous humic-like component. A significant relationship between the indirect photodegradation of SD and the decay of DOM fluorescent components was found (correlation coefficient, 0.99), and the different indirect photodegradation of SD in various DOM solutions might be ascribed to the different components of DOM. The indirect photolysis rate of SD first increased and then decreased with increasing pH. SD photolysis was enhanced by low salinity but remained stable at high salinity. The increased carbonate concentration inhibited SD photolysis, whereas nitrate showed almost no effect in this study. (C) 2020 Elsevier Ltd. All rights reserved.
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