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Occurrence, source and ecotoxicological risk assessment of pesticides in surface water of Wujin District (northwest of Taihu Lake), China

文献类型： 外文期刊

作者： Zhou, Yitong 1 ; Wu, Junxue 2 ; Wang, Bin 2 ; Duan, Lei 2 ; Zhang, Yizhe 2 ; Zhao, Wenxing 2 ; Wang, Fang 2 ; Sui, Qian 5 ;

作者机构： 1.Hebei Univ Engn, Coll Energy & Environm Engn, Handan 056038, Peoples R China

2.Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing Key Lab Emerging Organ Contaminants Contr, Beijing 100084, Peoples R China

3.Beijing Acad Agr & Forestry Sci, Inst Plant & Environm Protect, Beijing 100097, Peoples R China

4.Res Inst Environm Innovat Suzhou, Suzhou 215163, Peoples R China

5.East China Univ Sci & Technol, Sch Resources & Environm Engn, Shanghai 200237, Peoples R China

6.South China Inst Environm Sci, State Environm Protect Key Lab Water Environm Sim, Minist Ecol & Environm, Guangzhou 510655, Peoples R China

7.Changzhou Environm Monitoring Ctr Jiangsu Prov, Changzhou 213001, Peoples R China

关键词： Pesticides; Occurrence; Taihu lake; Surface water; Ecotoxicological risk

期刊名称：ENVIRONMENTAL POLLUTION （ 影响因子：8.071； 五年影响因子：8.35 ）

ISSN： 0269-7491

年卷期： 2020 年 265 卷

页码：

收录情况： SCI

摘要： This study investigated the occurrence and distribution of pesticides in surface water (lakes, major rivers and tributaries) and potential discharge sources (fish ponds, livestock and poultry farms, and sewage treatment plants) in Wujin District (northwest of Taihu Lake), Jiangsu province, China. An analytical liquid chromatography-tandem mass spectrometry method was developed for 38 pesticides, which was applied in the monitoring of 240 surface water samples and 76 potential discharge source samples. Eleven insecticides and five fungicides with temporal and spatial variation were detected in surface water. The total pesticide concentrations in surface water in different seasons were as follows: March > August > June > November. The two most polluting and widespread pesticides were carbendazim (maximum concentration 508 ng L-1, detection rate 100%) and imidacloprid (maximum concentration 438 ng L-1, detection rate 88%). Gehu Lake (S46) and Sanshangang River (S12) were seriously polluted water bodies. Seven insecticides and four fungicides were detected in the potential discharge sources; and their composition changed significantly with the seasons. The concentrations of detected organophosphorus pesticides and neonicotinoids (e.g. acetamiprid in March and dichlorvos in November) in a few non-agricultural planting sources were far greater than those detected in surface water, and hence a few fish ponds, livestock and poultry farms, and sewage treatment plants might be the potential discharge sources of pesticides in the surrounding surface water. The estimated input flux of the studied pesticides from upstream rivers to Taihu Lake was 141.95 kg a(-1). Furthermore, more attention should be paid to the medium or high aquatic ecotoxicological risk presented by the levels of organophosphorus pesticides, carbamates, and benzimidazoles. (C) 2020 Elsevier Ltd. All rights reserved.

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