Visible-light driven tetracycline hydrochloride degradation by nano-lanthanum hydroxide modified carbon nitride: performance, mechanism, and application in real wastewater treatment
文献类型： 外文期刊
作者： Xiong, Jian 1 ; Xu, Hanghang 1 ; Yin, Xuejie 2 ; Yang, Bei 2 ; Petropoulos, Evangelos 3 ; Xue, Lihong 2 ; Yang, Linzhang 2 ; He, Shiying 2 ;
作者机构： 1.Henan Univ Sci & Technol, Coll Chem & Chem Engn, 263, Kaiyuan Ave, Luoyang, Henan, Peoples R China
2.Inst Agr Resources & Environm, Jiangsu Acad Agr Sci, Key Lab Agroenvironm Downstream Yangtze Plain, Minist Agr, 50, Zhongling St, Nanjing, Jiangsu, Peoples R China
3.Newcastle Univ, Sch Engn, Newcastle Upon Tyne NE1 3DY, El Salvador
4.Stantec, Newcastle Upon Tyne NE1 3DY, England
期刊名称：ENVIRONMENTAL SCIENCE-WATER RESEARCH & TECHNOLOGY （ 影响因子：5.0； 五年影响因子：5.2 ）
ISSN： 2053-1400
年卷期： 2023 年 9 卷 8 期
页码：
收录情况： SCI
摘要： In this study, La(OH)(3)/g-C3N4 photocatalyst was designed for degradation of tetracycline hydrochloride (TCH) under visible light. The impact of different operational factors (dosage, initial TCH concentration, photocatalytic time, temperature, and competing anions and organic matter) on the removal of TCH was analyzed. La(OH)(3)/g-C3N4 exhibits a narrowed bandgap (2.90 eV) and enhanced visible-light absorption, leading to efficient TCH degradation (90.1%) and excellent reuse potential. The degradation intermediates were analyzed by liquid chromatography-mass spectrometry (LC-MS) to deduce the plausible degradation pathways. Quantitative structure activity relationship (QSAR) assessment indicated that the toxicity of the degradation products was greatly reduced. Furthermore, La(OH)(3)/g-C3N4 can simultaneously remove TCH, COD and PO43- from real wastewater by 56.31%, 69.63% and 89.9% respectively, demonstrating its robust potential in water and wastewater engineering and science.
- 相关文献
作者其他论文 更多>>
-
Efficient magnetic capture of PE microplastic from water by PEG modified Fe3 O4 nanoparticles: Performance, kinetics, isotherms and influence factors
作者：Zhang, Yifan;Feng, Yanfang;Xue, Lihong;He, Shiying;Zhang, Yifan;Duan, Jingjing;Liu, Ruiqian;Feng, Yanfang;Xue, Lihong;Yang, Linzhang;He, Shiying;Petropoulos, Evangelos;Petropoulos, Evangelos
关键词：Microplastic removal; Adsorption; Magnetic nanoparticles; Wastewater; Surface modification
-
Under what circumstances can chemical oxidation processes effectively degrade antibiotics resistance genes? Evidence from meta-analysis
作者：Ren, Zhuo;Ma, Xijun;Zhang, Jing;Ren, Zhuo;Yang, Bei;Hou, Pengfu;He, Shiying;Xue, Lihong;Yang, Linzhang;Petropoulos, Evangelos;Petropoulos, Evangelos;Liu, Hao
关键词：Chemical oxidation processes; Degradation; Antibiotics resistance genes; Meta -analysis
-
Floating La modified g-C3N4 photocatalytic sponge mesh for sustainable dye degradation under sunlight irradiation
作者：Xu, Hanghang;Xiong, Jian;Xu, Hanghang;Zhang, Yifang;Cheng, Jiahui;Yang, Bei
关键词：Nanoparticles; Nanocomposites; Photocatalytic sponge mesh; Immobilization; Dye degradation
-
A low-methane rice with high-yield potential realized via optimized carbon partitioning
作者：Hu, Jia;Bettembourg, Mathilde;Sun, Chuanxin;Jin, Yunkai;Sundstrom, Jens F.;Schnurer, Anna;Xue, Lihong;Hu, Ronggui
关键词：Global warming; Rice cultivars; Carbon partitioning; Methane emission; Agronomic practices; Root exudates
-
Sustainable design of photo-Fenton-like oxidation process in actual livestock wastewater through the highly dispersed FeCl 3 anchoring on a g-C 3 N 4 substrate
作者：Feng, Yanfang;Liang, Yunyi;Ding, Chenman;Jin, Hongmei;He, Shiying;Xue, Lihong;Liang, Yunyi;Xia, Changlei;Jiang, Yue;Rong, Shaopeng;Wu, Jun
关键词：Photo-Fenton-Like catalysis; Actual livestock wastewater; Outdoor device; Life cycle assessment; Products toxicity
-
Manure derived hydrochar reduced phosphorus loss risk via an alteration of phosphorus fractions and diversified microbial community in rice paddy soil
作者：Ding, Shudong;Li, Jing;He, Shiying;Xie, Huifang;Fu, Haibin;Feng, Yanfang;Xue, Lihong;Wang, Yu;Xie, Huifang;Fu, Haibin;Shaheen, Sabry M.;Rinklebe, Joerg;Shaheen, Sabry M.;Shaheen, Sabry M.
关键词：Hydrothermal carbonization; P speciation in paddy soils; 31P liquid NMR; Microbial community; Network diagram analysis
-
Unravelling superior photodegradation ability and key photoactive structures of hydrochar particle to typical emerging contaminant than corresponding bulk hydrochar from food waste
作者：Guo, Wenjing;Zhang, Zhiyong;Feng, Yanfang;He, Shiying;Fang, Guodong;Rong, Shaopeng
关键词：Hydrochar; Norfloxacin; Electron-hole; Graphitic-N; Density functional theory
