Isopropanol thermal treatment strategy for enhancing commercial nanofiltration membrane performance: High selectivity and superior antifouling capability
文献类型： 外文期刊
作者： Huang, Weiwei 1 ; Wang, Lin 3 ; Zhou, Wenzong 1 ; Lv, Weiwei 1 ; Yuan, Quan 1 ; Yang, Hang 1 ; Kang, Xinwei 4 ; Wu, Daoji 3 ; Zhu, Xuewu 3 ;
作者机构： 1.Shanghai Acad Agr Sci, Ecoenvironm Protect Res Inst, Lab Integrated Rice Fish Farming Ecosyst, Minist Agr & Rural Affairs, Shanghai 201403, Peoples R China
2.Shanghai Engn Res Ctr Low Carbon Agr, Shanghai 201403, Peoples R China
3.Shandong Jianzhu Univ, Sch Municipal & Environm Engn, Jinan 250101, Peoples R China
4.Ningbo RXHL Technol Co Ltd, Ningbo 315312, Peoples R China
关键词： Commercial nanofiltration membranes; Isopropanol (IPA) thermal treatment; Minerals/organic matter selectivity; Anti-fouling
期刊名称：JOURNAL OF MEMBRANE SCIENCE （ 影响因子：9.0； 五年影响因子：8.8 ）
ISSN： 0376-7388
年卷期： 2025 年 735 卷
页码：
收录情况： SCI
摘要： Commercial nanofiltration (NF) membranes face significant challenges including low permeate flux, membrane fouling, and difficulty in precisely tuning separation selectivity. This study presents an innovative isopropanol (IPA) thermal treatment strategy for optimizing commercial NF270 membrane performance. Through systematic characterization, we demonstrate that IPA molecules penetrate polyamide molecular chain interstices, weakening intermolecular interactions through solvation effects to achieve controllable crosslinking reduction from 60.4 % to 20.3 %. The de-crosslinking processes significantly improved surface hydrophilicity and enhanced surface negativity. The optimized NF-IPA/60 membrane exhibited high permeance (26.7 LMH/bar) and excellent Na2SO4 rejection (>95.7 %) while achieving enhanced selectivity for monovalent species. When treating natural surface water, NF-IPA/60 demonstrated superior contaminant removal and mineral retention capabilities, achieving >80.2 % organic contaminant removal while allowing moderate passage of beneficial minerals (Ca2+, Mg2+). Additionally, the membrane exhibited exceptional antifouling performance with flux recovery ratios exceeding 91.7 % throughout three fouling cycles, attributed to synergistic effects of enhanced surface charge, improved hydrophilicity, and reduced surface roughness. This approach provides a facile, environmentally friendly pathway for developing high-performance NF membranes with tailored separation characteristics for advanced water treatment applications.
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