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Polybrominated diphenyl ethers and novel brominated flame retardants in indoor dust of different microenvironments in Beijing, China

文献类型： 外文期刊

作者： Bu, Qingwei 1 ; Wu, Dongkui 1 ; Xia, Jing 2 ; Wu, Min 2 ; Liu, Xiaotu 2 ; Cao, Zhiguo 5 ; Yu, Gang 2 ;

作者机构： 1.China Univ Min & Technol Beijing, Sch Chem & Environm Engn, Beijing 100083, Peoples R China

2.Tsinghua Univ, Beijing Key Lab Emerging Organ Contaminants Contr, State Key Joint Lab Environm Simulat & Pollut Con, Sch Environm, Beijing 100084, Peoples R China

3.Beijing Res Ctr Agr Stand & Testing, 9 Middle Rd Shuguanghuayuan, Beijing 100097, Peoples R China

4.Jinan Univ, Sch Environm, Guangzhou 510632, Guangdong, Peoples R China

5.Henan Norma

关键词： Brominated flame retardants (BFRs); Floor dust; Elevated surface dust; Human exposure; Toddlers; Day care centers

期刊名称：ENVIRONMENT INTERNATIONAL （ 影响因子：9.621； 五年影响因子：10.72 ）

ISSN： 0160-4120

年卷期： 2019 年 122 卷

页码：

收录情况： SCI

摘要： The occurrence levels of eight polybrominated diphenyl ethers (PBDEs) and four novel brominated flame retardants (NBFRs) were determined and compared in indoor dust from different microenvironments (21 homes, 23 offices and 16 day care centers) in Beijing, China. Concentrations of Sigma 8PBDEs in dust were 430-17,000 ng/g, 690-8600 ng/g, and 90-2300 ng/g for homes, offices, and day care centers, respectively, and were dominated by BDE-209. Concentrations of Sigma(4)NBFRs ranged from 310 to 17,000 ng/g, 300 to 4300 ng/g, and not detected to 500 ng/g for homes, offices, and day care centers, respectively, and were dominated by bis(2-ethylhexyl)3,4,5,6-tetrabromophthalate (BEH-TEBP) and decabromodiphenylethane (DBDPE) across microenvironments. The results showed an increasing detection and elevated concentration of NBFRs (especially BEH-TEBP), indicating that monitoring of NBFRs in dust samples should be of concern in future studies. A notable finding was that the BFR concentrations in dust samples from day care centers were generally one order of magnitude lower than those from homes and offices in the present study. This implies that previous estimates of toddler exposure via dust ingestion on data from homes may be overestimated. Concentrations of BDE-209 and Sigma 8PBDEs were found to be significantly higher in elevated surface dust than floor dust from day care centers. The estimates of daily intakes of BFRs via dust ingestion for Chinese adults and toddlers using Monte Carlo analysis were 2-5 orders of magnitude lower than the corresponding reference daily intakes.

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