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Preliminary release inventories of unintentionally generated dl-PCB and HCB from sources in China: Base year 2015

文献类型： 外文期刊

作者： Chen, Ping 1 ; Gong, Wenwen 1 ; Yu, Gang 1 ; Fiedler, Heidelore 1 ;

作者机构： 1.Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut Con, Beijing Key Lab Emerging Organ Contaminants Contr, Sch Environm, Beijing 100084, Peoples R China

2.Beijing Acad Agr & Forestry Sci, Beijing Res Ctr Agr Stand & Testing, Beijing 100097, Peoples R China

3.Orebro Univ, Sch Sci & Technol, MTM Res Ctr, SE-70182 Orebro, Sweden

关键词： Dioxin-like polychlorinated biphenyls; Hexachlorobenzene; Release inventory for China; Toolkit methodology under the Stockholm; convention on persistent organic pollutants

期刊名称：CHEMOSPHERE （ 影响因子：7.086； 五年影响因子：6.956 ）

ISSN： 0045-6535

年卷期： 2019 年 219 卷

页码：

收录情况： SCI

摘要： This research presents release inventories of unintentionally generated dioxin-like polychlorinated biphenyls (dl-PCB) and hexachlorobenzene (HCB), which so far have not been developed or assessed. For the inventory development, the amended Toolkit methodology as developed for reporting under the Stockholm Convention on Persistent Organic Pollutants, has been applied. Based on the activity rate (AR) obtained from various statistical yearbooks, reports, or scientific literature, and the emission factors (EFs) suited to each technology level, we estimated the preliminary release inventories of unintentionally produced dl-PCB and HCB from 36 source categories in China for the reference year 2015. The result showed that in 2015, 656 g TEQ of unintentionally produced dl-PCB and 2,145,504 g (or 2146 kg) of unintentionally generated HCB were released in China from these 36 source categories. Most of dl-PCB and HCB was released to air, 71% or 60%, respectively. For comparison and for the sources which could be estimated for all three unintentional POPs the total releases of PCDD/PCDF were 5695 g TEQ per year. Of these, 78% were released to air. For dl-PCB and HCB, the vast majority of the releases from the source group 7 Production and use of consumer goods - is found in the products and not in air. With respect to source attribution and releases to air, the source groups SG3 - Heat and power generation and SG2 - Ferrous and non-ferrous metal production dominate the air emission inventory. Due to the lack of EFs, the calculated releases to the water and land were not well covered, which overall results in an underestimation of the total releases for all unintentional POPs. For comparison, the release inventories from Japan and from several other countries that were developed using methodologies other than the UNEP Toolkit are presented as well. (C) 2018 Elsevier Ltd. All rights reserved.

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