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Long-term effects of sediment dredging on controlling cobalt, zinc, and nickel contamination determined by chemical fractionation and passive sampling

文献类型： 外文期刊

作者： Chen, Musong 1 ; Ding, Shiming 1 ; Gao, Shuaishuai 1 ; Xu, Shiwei 3 ; Yang, Chenye 3 ; Wu, Yuexia 1 ; Gong, Mengdan 4 ; W 1 ;

作者机构： 1.Chinese Acad Sci, Nanjing Inst Geog & Limnol, State Key Lab Lake Sci & Environm, Nanjing 210008, Jiangsu, Peoples R China

2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China

3.Jiangsu Acad Agr Sci, Cent Lab, Nanjing 210008, Jiangsu, Peoples R China

4.Shanghai Water Source Construct Dev Co Ltd, Shanghai 200437, Peoples R China

5.Shanghai Waterway Engn Design & Consulting Co Ltd, Shanghai 200120, Peoples R China

6.Nanjing EasySensor Environm Technol Co Ltd

关键词： Sediments; Dredging project; Heavy metals; In-situ monitoring; Algal blooms

期刊名称：CHEMOSPHERE （ 影响因子：7.086； 五年影响因子：6.956 ）

ISSN： 0045-6535

年卷期： 2019 年 220 卷

页码：

收录情况： SCI

摘要： Studies of dredging effectiveness, especially the ones that last for several years, are scarce. In this study, we evaluated effectiveness of dredging performed for six years on controlling cobalt (Co), zinc (Zn), and nickel (Ni) contamination of sediments. High-resolution dialysis (HR-Peeper) and diffusive gradients in thin films (DGT) methods were applied to analyze the non-dredged and post-dredging sediments. The soluble and DGT-labile Co and Ni content declined by 22% and 44% (soluble) and by 16% and 26% (labile) in April, July and October in the post-dredging region. In contrast, their concentrations increased by 105% and 9% (soluble) and 322% and 27% (labile) in January. These changes in the dredging effects were caused by the corresponding changes in the reducible and residual fractions of Co and the residual fraction of Ni in sediments in the dredged site, respectively. Soluble and DGT-labile Zn decreased on average by 23% and 29% in July and October and increased on average by 151% and 52% in April and January in the post dredging region. The different Zn mobility in the post-dredging region was controlled by the reducible fraction of Zn. The results revealed positive influence of dredging engineering in summer, autumn and/or spring and negative one in winter. Therefore, an accurate assessment of dredging effectiveness should take its seasonal variation into consideration. (C) 2018 Elsevier Ltd. All rights reserved.

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