Preparation of nitrogen-doped bagasse-derived biochar with outstanding methylene blue adsorption performance
文献类型： 外文期刊
作者： Cai, Faming 1 ; Li, Cunjun 1 ; Yang, Chenghu 2 ; Wang, Yuying 2 ; Zhou, Hanghai 2 ; Yang, Shengmao 2 ; Tang, Jiangwu 2 ; Wang, Linjiang 1 ; Liu, Yuxue 1 ;
作者机构： 1.Guilin Univ Technol, Coll Mat Sci & Engn, Key Lab New Proc Technol Nonferrous Met & Mat, Guangxi Key Lab Opt & Elect Mat & Devices,Minist E, Guilin 541004, Peoples R China
2.Zhejiang Acad Agr Sci, Inst Environm Resource Soil & Fertilizer, State Key Lab Managing Biot & Chem Threats Qual &, Hangzhou 310021, Peoples R China
3.Guilin Univ Technol, Collaborat Innovat Ctr Explorat Nonferrous Met Dep, Guilin 541004, Peoples R China
4.Engn Res Ctr Biochar Zhejiang Prov, Hangzhou 310021, Peoples R China
关键词： Carbon-based material; Porous structure; Nitrogen doping; Chemical activation; Organic dyes; Adsorption mechanism
期刊名称：INDUSTRIAL CROPS AND PRODUCTS （ 影响因子：6.2； 五年影响因子：6.2 ）
ISSN： 0926-6690
年卷期： 2025 年 224 卷
页码：
收录情况： SCI
摘要： Biochar is a promising adsorbent for wastewater treatment; however, effective modification techniques are required to optimize its adsorption efficiency. In this study, nitrogen-doped modified bagasse biochar was prepared from bagasse biomass using a synchronous pyrolysis and activation process with urea (CH4N2O) as the N source and sodium bicarbonate (NaHCO3) as the chemical activator. Adsorption experiments of the modified sugarcane bagasse biochar for removing methylene blue (MB) in aqueous solution were carried out to investigate the effects of different biochar dosages, solution pH, and adsorption time on the adsorption performance. Adsorption optimization experiments reveal that the adsorption capacity of 50 mg modified biochar added to a 30 mg/L MB solution at 40 degrees C and pH 11.0 is similar to 20 times that of unmodified biochar at the same dose after 120 min (84.2 and 4.45 mg/g, respectively). The isothermal adsorption behavior of MB with the biochar conforms to the Langmuir model and the adsorption kinetics follows the quasi-second-order kinetic equation, indicating that chemical adsorption dominates such adsorption. The adsorption performance of the biochar before and after modification were characterized using scanning electron microscopy, Fourier-transform infrared spectroscopy, X-ray photoelectron spectroscopy, and elemental analysis to explore the adsorption mechanism. This study increases the scope for the disposal and utilization of bagasse agricultural waste and has important practical significance for the development of low-cost environmentally-friendly adsorbent materials.
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