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Identification and visualization of environmental microplastics by Raman imaging based on hyperspectral unmixing coupled machine learning

文献类型： 外文期刊

作者： Li, Fang 1 ; Liu, Dongsheng 2 ; Guo, Xuetao 3 ; Zhang, Zhenming 4 ; Martin, Francis L. 5 ; Lu, Anxiang 1 ; Xu, Li 1 ;

作者机构： 1.Beijing Acad Agr & Forestry Sci, Inst Qual Stand & Testing Technol, Beijing 100095, Peoples R China

2.Beijing Acad Agr & Forestry Sci, Inst Plant Nutr Resources & Environm, Beijing 100097, Peoples R China

3.Northwest A&F Univ, Coll Nat Resources & Environm, Yangling 712100, Shaanxi, Peoples R China

4.Guizhou Univ, Coll Resource & Environm Engn, Guiyang 550003, Guizhou, Peoples R China

5.Biocel Ltd, Kingston Upon Hull HU10 6TS, England

6.Blackpool Teaching Hosp NHS Fdn Trust, Dept Cellular Pathol, Whinney Heys Rd, Blackpool FY3 8NR, England

关键词： Microplastic; Raman imaging; Alternating volume maximization; Hyperspectral unmixing; Machine learning

期刊名称：JOURNAL OF HAZARDOUS MATERIALS （ 影响因子：13.6； 五年影响因子：12.7 ）

ISSN： 0304-3894

年卷期： 2024 年 465 卷

页码：

收录情况： SCI

摘要： Microplastics (MPs) are ubiquitous contaminants that have become an emerging pollutant of concern, potentially threatening human health and ecosystem environments. Although current detection methods can accurately identify various types of MPs, it remains necessary to develop non-destructive and rapid methods to meet growing demands for detection. Herein, we combine a hyperspectral unmixing method and machine learning to analyse Raman imaging data of environmental MPs. Five MPs types including poly(butylene adipate-coterephthalate) (PBAT), poly(butylene succinate) (PBS), p-polyethylene (PE), polystyrene (PS) and polypropylene (PP) were visualized and identified. Individual or mixed pure or aged MPs along with environmental samples were analysed by Raman imaging. Alternating volume maximization (AVmax) combined with unconstrained least squares (UCLS) method estimated end members and abundance maps of each of the MPs in the samples. Pearson correlation coefficients (r) were used as the evaluation index; the results showed that there is a high similarity between the raw spectra and the average spectra calculated by AVmax. This indicates that Raman imaging based on machine learning and hyperspectral unmixing is a novel imaging analysis method that can directly identify and visualize MPs in the environment.

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