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Polycyclic Aromatic Hydrocarbons (PAHs) in Exposed-Lawn Soils from 28 Urban Parks in the Megacity Guangzhou: Occurrence, Sources, and Human Health Implications

文献类型: 外文期刊

作者: Ke, Chang-Liang 1 ; Gu, Yang-Guang 1 ; Liu, Qi 1 ;

作者机构: 1.Chinese Acad Fishery Sci, South China Sea Fisheries Res Inst, Guangzhou 510300, Guangdong, Peoples R China

2.Guangdong Prov Key Lab Fishery Ecol & Environm, Guangzhou 510300, Guangdong, Peoples R China

3.Minist Agr, Key Lab South China Sea Fishery Resources Exploit, Guangzhou 510300, Guangdong, Peoples R China

期刊名称:ARCHIVES OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY ( 影响因子:2.804; 五年影响因子:3.399 )

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收录情况: SCI

摘要: Polycyclic aromatic hydrocarbons (PAHs) in urban soils may pose a serious threat to human health via oral ingestion, dermal absorption, and particulate inhalation, especially in public parks and playgrounds, with children and senior citizens showing the highest susceptibility. Several studies have been undertaken identifying PAHs in urban soils, but no studies to date have assessed PAHs in urban parks, in particular in exposed-lawn soils. In recent decades, unprecedented rates of urbanization and industrialization in China have resulted in significant levels of urban environmental pollution. However, concentrations, sources, and the health risk associated with PAH exposure via urban park lawn soils in China remain unknown. The concentrations, sources, and health risk of exposure to 16 PAHs in surface-exposed lawn soils were studied in 28 urban parks in Guangzhou. Concentrations of Sigma 16PAHs ranged from 76.44 to 890.85 ng/g with a mean of 286.11 ng/g. PAH composition was mostly characterized by 2- and 4-ring PAHs in most sampling parks; Nap, Flua, Pyr, Phe, and Chr were the dominant constituents. Principle component analysis coupled with multivariate linear regression indicated that vehicular and coal combustion emissions contributed to 50.53 and 49.46% of PAHs in Guangzhou's urban park soils, respectively. Total cancer risk (TCR) analysis found that 22 parks (accounting for 78.57% total parks) designed for children's use and general-use park areas presented a potentially high risk (> 1 x 10(-4)) for all users.

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