Enhanced ammonium removal on biochar from a new forestry waste by ultrasonic activation: Characteristics, mechanisms and evaluation
文献类型： 外文期刊
作者： Wang, Tongtong 1 ; Li, Gaoliang 2 ; Yang, Kaiqi 1 ; Zhang, Xiaoyuan 1 ; Wang, Ke 1 ; Cai, Jinjun 1 ; Zheng, Jiyong 1 ;
作者机构： 1.Northwest A&F Univ, Coll Nat Resources & Environm, State Key Lab Soil Eros & Dryland Farming Loess P, Yangling 712100, Shaanxi, Peoples R China
2.Chinese Acad Sci & Minist Water Resources, Inst Soil & Water Conservat, Yangling 712100, Shaanxi, Peoples R China
3.Ningxia Acad Agr & Forestry Sci, Inst Resources & Environm, Yinchuan 750002, Ningxia, Peoples R China
关键词： Caragana korshinskii biochar; Ultrasonic activation; Adsorption characteristics; Mechanisms; Ammonium
期刊名称：SCIENCE OF THE TOTAL ENVIRONMENT （ 影响因子：7.963； 五年影响因子：7.842 ）
ISSN： 0048-9697
年卷期： 2021 年 778 卷
页码：
收录情况： SCI
摘要： The adsorption treatment of ammonium-containing wastewater has attracted significant global attention. Most enhanced adsorption methods employ chemical modification, and there are few reports on physical activation. We present a physical activation to explore whether physical ultrasound may enhance the adsorption performance and comprehensive utilisation of a new forestry waste, Caragana korshinskii was used as a feedstock to prepare activated biochar (ACB) by controlling the pyrolysis temperatures and ultrasound parameters. The optimal parameters were determined via batch adsorption of NH4+, and the adsorption characteristics were assessed by 8 kinds of models and influence experiments. Moreover, the physicochemical properties of ACB during the pyrolysis process were investigated, and the ultrasonic activation and adsorption mechanisms were discussed using multiple characterisation techniques. Additionally, the cost analysis, the safety of the ultrasonic process and disposal method also were evaluated. The results showed that the ultrasonic activation significantly enhanced the NH4+ adsorption efficiency of biochar by approximately 5 times. ACB exhibited the best performance at 500 degrees C with an ultrasonic activation time of 480 min, frequency of 45 kHz, and power of 700 W. The ultrasonic activation reduced the biochar ash and induced pore formation, which increased the specific surface area through cavitation corrosion and micro-acoustic flow mechanism. The NH4+ adsorption mechanisms comprised physicochemical processes, of which physical adsorption was dominant. The preparation cost of 1 kg ACB was about 0.42 US dollar, and no secondary pollution occurred in the activation process. The findings prove that ultrasonic technology is efficient and convenient for enhancing biochar adsorption performance, and thus is suitable for industrial applications and promotion. (C) 2021 Elsevier B.V. All rights reserved.
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