Streamlined Synthesis of Ga-Cu Dual Single-Atom Nanozymes for Advanced Electrochemical Sensing Applications
文献类型： 外文期刊
作者： Song, Guangchun 1 ; Zheng, Xiaochun 1 ; Zhang, Zedong 3 ; Fauconnier, Marie-Laure 2 ; Li, Cheng 1 ; Chen, Li 1 ; Zhang, Dequan 1 ;
作者机构： 1.Chinese Acad Agr Sci, Inst Food Sci & Technol, Key Lab Agroprod Qual & Safety Control Storage & T, Minist Agr & Rural Affairs, Beijing 100193, Peoples R China
2.Univ Liege, Lab Chem Nat Mol, Gembloux Agrobio Tech, Passage Deportes 2, B-5030 Gembloux, Belgium
3.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
关键词： dual single-atom nanozymes; electrochemical sensors; hydrotalcite carrier; meat freshness monitoring
期刊名称：ADVANCED FUNCTIONAL MATERIALS （ 影响因子：19.0； 五年影响因子：19.4 ）
ISSN： 1616-301X
年卷期： 2025 年
页码：
收录情况： SCI
摘要： The real-time, rapid, and portable detection of food freshness is crucial for assessing food quality and ensuring food safety. Volatile amines produced during food spoilage have significant potential as markers for evaluating freshness. In this study, an electrochemical sensing platform is developed for the detection of volatile amines using gallium-copper dual single-atom nanozymes (with Ga and Cu contents of 1.31and 4.07 wt.%, respectively) supported by a 2D layered double hydroxide (LDH). The synergistic loading of the dual atoms facilitated binding with volatile amines, which accelerated electron transfer at the GaCu-LDH surface, inducing changes in the electrical signals and enabling detection. The platform exhibited a rapid response time of approximate to 4 s, with a good linear relationship between the ammonia concentration and steady-state current within the range of 0.05-0.4 mm and a detection limit of 5.9 mu m. This electrochemical sensor platform enabled the rapid, portable, and intelligent detection and monitoring of the freshness of meat from livestock and poultry (pork, beef, lamb, and chicken) at room temperature and under refrigerated storage conditions, providing a valuable method for the real-time monitoring of food freshness.
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