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Chinese coastal seas are facing heavy atmospheric nitrogen deposition

文献类型: 外文期刊

作者: Luo, X. S. 1 ; Tang, A. H. 1 ; Shi, K. 3 ; Wu, L. H. 4 ; Li, W. Q. 5 ; Shi, W. Q. 6 ; Shi, X. K. 7 ; Erisman, J. W. 8 ; Zhan 1 ;

作者机构: 1.China Agr Univ, Coll Resources & Environm Sci, Beijing 100094, Peoples R China

2.Henan Acad Agr Sci, Inst Plant Nutr Resources & Environm Sci, Zhengzhou, Peoples R China

3.Dalian Jiaotong Univ, Coll Environm & Chem Engn, Dalian, Peoples R China

4.Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou 310003, Zhejiang, Peoples R China

5.Fujian Inst Tobacco Agr Sci, Fuzhou, Peoples R China

6.Chinese Acad Trop Agr Sci, South Subtrop Crops Res Inst, Zhanjiang, Peoples R China

7.Agr Forestry & Water Dept Changdao Cty, Changdao, Peoples R China

8.Louis Bolk Inst, NL-3972 LA Driebergen, Netherlands

关键词: reactive N;atmospheric deposition;coastal sea;eutrophication;China

期刊名称:ENVIRONMENTAL RESEARCH LETTERS ( 影响因子:6.793; 五年影响因子:7.801 )

ISSN: 1748-9326

年卷期: 2014 年 9 卷 9 期

页码:

收录情况: SCI

摘要: As the amount of reactive nitrogen (N) generated and emitted increases the amount of N deposition and its contribution to eutrophication or harmful algal blooms in the coastal zones are becoming issues of environmental concern. To quantify N deposition in coastal seas of China we selected six typical coastal sites from North to South in 2011. Concentrations of NH3, HNO3, NO2, particulate NH4+ (pNH(4)(+)) and pNO(3)(-) ranged from 1.97-4.88, 0.46-1.22, 3.03-7.09, 2.24-4.90 and 1.13-2.63 mu g Nm(-3) at Dalian (DL), Changdao (CD), Linshandao (LS), Fenghua (FH), Fuzhou (FZ), and Zhanjiang (ZJ) sites, respectively. Volume-weighted NO3--N and NH4+-N concentrations in precipitation varied from 0.46 to 1.67 and 0.47 to 1.31 mg N L-1 at the six sites. Dry, wet and total deposition rates of N were 7.8-23.1, 14.2-25.2 and 22.0-44.6 kg N ha(-1) yr(-1) across the six coastal sites. Average N dry deposition accounted for 45.4% of the total deposition and NH3 and pNH(4)(+) contributed to 76.6% of the dry deposition. If we extrapolate our total N deposition of 33.9 kg N ha(-1) yr(-1) to the whole Chinese coastal sea area (0.40 million km(2)), total N deposition amounts to 1.36 Tg N yr(-1), a large external N input to surrounding marine ecosystems.

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