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Carbon-14 labeled transformation of atrazine in soils: Comparison of superabsorbent hydrogel coating and technical material

文献类型： 外文期刊

作者： Cheng, Xi 1 ; Yang, Jingying 3 ; Zhang, Chunrong 1 ; Tang, Tao 1 ; Zhao, Xueping 1 ; Ye, Qingfu 2 ;

作者机构： 1.Zhejiang Acad Agr Sci, State Key Lab Managing Biot & Chem Threats Qual &, Key Lab Pesticide Residue Detect, Minist Agr & Rural Affairs,Inst Agroprod Safety &, Hangzhou 310021, Peoples R China

2.Zhejiang Univ, Inst Nucl Agr Sci, Key Lab Nucl Agr Sci, Minist Agr & Rural Affairs, Hangzhou 310058, Peoples R China

3.Pharmaron Ningbo Technol Dev Co Ltd, Radiolabeled DMPK & BA Lab, Ningbo 315336, Peoples R China

关键词： Superabsorbent hydrogel; Atrazine; Soil; Fate model; Degradation

期刊名称：SCIENCE OF THE TOTAL ENVIRONMENT （ 影响因子：8.2； 五年影响因子：8.6 ）

ISSN： 0048-9697

年卷期： 2024 年 951 卷

页码：

收录情况： SCI

摘要： Atrazine exhibits adverse effects on diverse organisms in both terrestrial and aquatic environments, even though it effectively targets specific organisms. This study employed superabsorbent hydrogels to coat 14C-atrazine coupled with a four-compartment model to determine the fate of this herbicide in three oxic soils over a 100-day incubation period. Mineralization of atrazine was limited in all soils, with rates remaining below 3.5 %. The encapsulation treatment reduced mineralization of atrazine in soil A and soil B. Bound residues ranged from 26.1 to 43.6% at 100 d. The encapsulation treatment enhanced the degradation of atrazine and reduced the content of deethylatrazine in soil A, but significantly increased the content of deisopropylatrazine in soil A and hydroxyatrazine in soil C. Using the obtained data, we also constructed a four-compartment model to clarify the relationships among the parent compound, degradation products, bound residues, and mineralization. This model accurately fits the fate of atrazine in the present work. Additionally, the correlation study suggested that both soil parameters and superabsorbent hydrogels played significant roles in influencing atrazine transformation. These findings serve as a reference for evaluating the environmental impact of superabsorbent hydrogels in atrazine pollution reduction and offer a foundational model approach for a comprehensive understanding of organic pollutants.

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