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Seasonal characteristics, source apportionment and ecological risk assessment of priority and emerging contaminants using passive samplers in the coastal water

文献类型: 外文期刊

作者: Diao, Zishan 1 ; Ping, Xianyin 3 ; Zhang, Xue 1 ; Hui, Bin 4 ; Zhu, Fanping 1 ; Zhang, Yiqiao 1 ; Wang, Jing 1 ; Yu, Yinjie 1 ; Zhang, Lin 1 ; Hui, Wenjia 5 ; Xie, Xiaomin 6 ; Zhang, Xiaohan 1 ; Wang, Shuguang 1 ; Yuan, Xianzheng 1 ;

作者机构: 1.Shandong Univ, Sch Environm Sci & Engn, Shandong Key Lab Water Pollut Control & Resource R, Qingdao 266237, Shandong, Peoples R China

2.Shandong Univ, Sch Environm Sci & Engn, Shandong Key Lab Environm Proc & Hlth, Qingdao 266237, Shandong, Peoples R China

3.Chinese Acad Fishery Sci, East China Sea Fisheries Res Inst, Shanghai 200090, Peoples R China

4.Qingdao Univ, Sch Mat Sci & Engn, Qingdao 266071, Shandong, Peoples R China

5.Shandong Univ, Weihai Inst Interdisciplinary Res, Weihai 264209, Shandong, Peoples R China

6.Qingdao Agr Univ, Coll Resources & Environm Sci, Qingdao 266109, Shandong, Peoples R China

7.Shandong Univ, WeiHai Res Inst Ind Technol, Shandong 264209, Peoples R China

关键词: Long-term monitoring; Diffusive gradients in thin-films (DGT); Polycyclic aromatic hydrocarbons (PAHs); Synthetic musks (SMs); Coastal waters

期刊名称:JOURNAL OF HAZARDOUS MATERIALS ( 影响因子:11.3; 五年影响因子:12.4 )

ISSN: 0304-3894

年卷期: 2025 年 493 卷

页码:

收录情况: SCI

摘要: The presence of priority and emerging contaminants in aquatic environments is a worldwide concern. This study utilized the diffusive gradients in thin-films (DGT) technique for in situ monitoring of polycyclic aromatic hydrocarbons (PAHs) and synthetic musks (SMs) in coastal waters over a year. DGT provided time-integrated and reliable pollutant measurements, outperforming grab sampling in terms of repeatability and stability. Seasonal and spatial variations in PAH and SM concentrations were observed, influenced by proximity to vehicle and maritime transport and tourist areas. Source apportionment using diagnostic ratios, positive matrix factorization, and principal component analysis indicated mixed pollutant origins. High ecological risks for certain PAHs emerged in the summer, highlighting significant seasonal threats. These findings provide critical insights for the long-term monitoring and management of PAHs and SMs, offering valuable regional data to support pollution mitigation efforts in the coastal water.

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