A novel PEI-grafted N-doping magnetic hydrochar for enhanced scavenging of BPA and Cr(VI) from aqueous phase?
文献类型： 外文期刊
作者： Qu, Jianhua 1 ; Bi, Fuxuan 1 ; Hu, Qi 2 ; Wu, Peipei 1 ; Ding, Boyu 1 ; Tao, Yue 1 ; Ma, Shouyi 3 ; Qian, Chunrong 4 ; Zhang, Ying 1 ;
作者机构： 1.Northeast Agr Univ, Sch Resources & Environm, Harbin 150030, Peoples R China
2.Shenyang Pharmaceut Univ, Sch Pharmaceut Engn, Shenyang 110016, Peoples R China
3.Heilongjiang Acad Land Reclamat Sci, Harbin 150030, Peoples R China
4.Heilongjiang Acad Agr Sci, Inst Crop Cultivat & Tillage, Harbin 150028, Peoples R China
关键词： Adsorption; N doping; PEI -Modification; Heavy metal; Organic pollutant
期刊名称：ENVIRONMENTAL POLLUTION （ 影响因子：8.9； 五年影响因子：9.5 ）
ISSN： 0269-7491
年卷期： 2023 年 321 卷
页码：
收录情况： SCI
摘要： Herein, polyethyleneimine (PEI)-grafted nitrogen-doping magnetic hydrochar (PEIMW@MNHC) was synthesized for hexavalent chromium (Cr(VI)) and bisphenol A (BPA) elimination from water. Characterizations exhibited that abundant amino functional groups, intramolecular heterocyclic N, azo and Fe-NX structures were successfully introduced into the inherent structure of hydrochar. The obtained PEIMW@MNHC presented maximum uptake of 205.37 and 180.79 mg/g for Cr(VI) and BPA, respectively, and was highly tolerant to various coexisting ions. Mechanism investigation revealed that the protonated amino, intramolecular heterocyclic N and Fe(II) participated in Cr(VI) reduction, and the N/O-containing groups and Fe(III) fixed Cr(III) onto PEIMW@MNHC by the formation of complexes and precipitates. On the other hand, azo, Fe-NX and graphitic N structures contributed to the removal of BPA via pore filling, hydrogen bonding and pi-pi interactions. Additionally, PEIMW@MNHC maintained over 85.0% removal efficiency for Cr(VI) and BPA after four cycles, manifesting that PEIMW@MNHC was an ideal adsorbent with outstanding practical application potential.
- 相关文献
作者其他论文 更多>>
-
Effects of depth of straw returning on maize yield potential and greenhouse gas emissions
作者：Wang, Junqiang;Han, Yehui;Zhou, Chao;Xu, Ting;Qu, Zhongcheng;Ma, Bo;Yuan, Ming;Wang, Lianxia;Liu, Yang;Li, Qingchao;Ma, Baoxin;Ding, Xinying;Qian, Chunrong
关键词：straw returning; maize; yield potential; greenhouse gases; soil organic carbon
-
Annual burying of pelletized straw benefits grain amino acid by increasing soil mineral elements: A case study in Northeast China
作者：Wang, Peixin;Wang, Xiquan;Wang, Xinbo;Pang, Huancheng;Wang, Peixin;Wang, Xiquan;Hao, Yubo;Zhang, Yiteng;Qian, Chunrong;Zong, Rui;Ni, Haiping;Liu, Lumin;Yang, Yan;Pang, Huancheng;Qian, Chunrong
关键词：Zea mays L.; Straw form; Straw returning; Soil mineral elements; Grain amino acid
-
Genome assembly of autotetraploid Actinidia arguta highlights adaptive evolution and enables dissection of important economic traits
作者：Lu, Xue-Mei;Yu, Xiao-Fen;Qu, Ming-Hao;Man, Yu-Ping;Jiang, Xiao-Han;Li, Mu-Zi;Wang, Jian;Chen, Qi-Qi;Lei, Rui;Zhao, Cheng-Cheng;Zhou, Yun-Qiu;Jiang, Zheng-Wang;Li, Zuo-Zhou;Li, Jie-Wei;Mo, Quan-Hui;Zhang, Ying;Lou, Xin;Peng, Hai-Xu;Yi, Ya-Ting;Wang, He-Xin;Zhang, Xiu-Jun;Li, Li;Zhang, Qiong;Gao, Lei;Wang, Yan-Chang;Li, Guo-Qiang;Lou, Xin;Wang, He-Xin;Wang, Yi-Bo;Qu, Ming-Hao;Jiang, Xiao-Han;Li, Mu-Zi;Zhou, Yun-Qiu;Peng, Hai-Xu;Yi, Ya-Ting;Wang, Huan;Zheng, Shang;Liu, Chuang;Dong, Chang;Wang, Bai-Lin;Sun, Yan-Xiang;Zhang, Hui-Qin;Li, Jie-Wei;Mo, Quan-Hui;Zhang, Ying;Lou, Xin;Wang, He-Xin;Peng, Hai-Xu;Yi, Ya-Ting;Wang, Dan;Wang, Wen-Xia;Liu, Yongbo;Gao, Lei;Wu, Jin-Hu
关键词：kiwiberry; dioecism; adaptive evolution; paleoclimate; GEA; rapid softening
-
Effects of Multi-Walled Carbon Nanotubes and Nano-Silica on Root Development, Leaf Photosynthesis, Active Oxygen and Nitrogen Metabolism in Maize
作者：Hao, Yubo;Yu, Yang;Gong, Xiujie;Jiang, Yubo;Lv, Guoyi;Zhang, Yiteng;Li, Liang;Zhao, Yang;Qian, Chunrong;Sun, Guangyan;Gu, Wanrong;Sun, Dan
关键词：maize; multi-walled carbon nanotubes; nano-silica
-
Climate-smart agriculture practice promotes sustainable maize production in northeastern China: Higher grain yield while less carbon footprint
作者：Feng, Xiaomin;Sun, Tao;Feng, Xiaomin;Sun, Tao;Deng, Aixing;Song, Zhenwei;Zhang, Weijian;Guo, Jinrui;Cai, Hongguang;Qian, Chunrong;Hao, Yubo;Yu, Yang;Song, Zhenwei
关键词：Integrated agronomic management; Soil organic carbon; Greenhouse gas mitigation; Carbon footprint; Net ecosystem economic benefit
-
Annual burying of straw after pelletizing: A novel and feasible way to improve soil fertility and productivity in Northeast China
作者：Wang, Xiquan;Zhang, Yan;Wang, Xinbo;Pang, Huancheng;Lv, Guoyi;Yu, Yang;Qian, Chunrong;Peixoto, Leanne
关键词：Zea mays L; Straw form; Straw returning; Soil nutrients; Crop yield
-
The association of social rank with paternity efficiency in competitive mating flocks of Zi goose ganders (Anser cygnoides L.) (vol 100, 101415, 2021)
作者：Zhang, Jiayue;Liu, Yang;Li, E.;Ning, Bolin;Zhang, Ying;Liu, Shengjun;Sun, Jinyan;Liu, Guojun
关键词：
