Light-Promoted Nickel-Catalyzed C-O/C-N Coupling of Aryl Halides with Carboxylic Acids and Sulfonamides
文献类型： 外文期刊
第一作者： Zhao, Tian-Tian
作者： Zhao, Tian-Tian;Qin, Hao-Ni;Xu, Peng-Fei;Xu, Peng-Fei
作者机构：
期刊名称：ORGANIC LETTERS （ 影响因子：5.2； 五年影响因子：4.9 ）
ISSN： 1523-7060
年卷期： 2023 年
页码：
收录情况： SCI
摘要： A general strategy for the construction of dual-functional carbon- heteroatom bonds has been developed via a light-promoted nickel catalytic system. Employing a simple NiBr2 as the catalyst without any exogeneous ligands and photosensitizers, a variety of esters and sulfonamide N-arylation derivatives, including celecoxib-and glimepiride-derived sulfonamides, were readily accessed with high functional group tolerance and high efficiency. Moreover, the UV-vis absorption spectrum and free radical trapping experiments aimed at revealing the mechanism of the reaction are also presented.
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