Behavior of tetracycline and macrolide antibiotics in activated sludge process and their subsequent removal during sludge reduction by ozone
文献类型： 外文期刊
作者： Wang, Lu 1 ; Ben, Weiwei 1 ; Li, Yangang 1 ; Liu, Chao 3 ; Qiang, Zhimin 1 ;
作者机构： 1.Chinese Acad Sci, Univ Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Key Lab Drinking Water Sci & Technol, 18 Shuang Qing Rd, Beijing 100085, Peoples R China
2.Chinese Acad Fishery Sci, Yellow Sea Fisheries Res Inst, Marine Fishery Environm & Bioremediat Lab, Qingdao 266071, Peoples R China
3.Clemson Univ, Dept Environm Engn & Earth Sci, Anderson, SC 29625 USA
关键词： Antibiotics; Sorption; Ozonation; Sludge reduction; Activated sludge process
期刊名称：CHEMOSPHERE （ 影响因子：7.086； 五年影响因子：6.956 ）
ISSN： 0045-6535
年卷期： 2018 年 206 卷
页码：
收录情况： SCI
摘要： Ozonation is a promising means for the reduction of excess sludge in wastewater treatment plants. However, little information is available on the removal of antibiotics during sludge ozonation. Therefore, this study investigated first the behavior of four commonly-used hydrophobic antibiotics, including three tetracyclines (tetracycline, oxytetracycline, and doxycycline) and one macrolide (azithromycin) in activated sludge process and then their removal during sludge reduction by ozone. Results indicate that the studied antibiotics were primarily transferred into the solid phase of activated sludge via sorption, which was a reversible, spontaneous, and exothermic process governed by surface reactions. Sludge ozonation could effectively remove 86.4-93.6% of the antibiotics present in the sludge at an ozone dose of 102 mg per gram of mixed liquor suspended solids and pH 7.2. The removal of studied antibiotics mainly proceeded through desorption and subsequent oxidation. Increasing the initial pH from 5.0 to 9.5 obviously enhanced the antibiotic removal during sludge ozonation. This study demonstrated that the activated sludge process coupled with sludge ozonation can simultaneously reduce excess sludge and eliminate antibiotics. (C) 2018 Elsevier Ltd. All rights reserved.
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