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High Quality Nitrogen and Silicon Co-Doped Carbon Dots (N/Si-CDs) for Fe3+ Sensing

文献类型： 外文期刊

作者： Wu, Jinzhu 1 ; Feng, Yaxiu 1 ; Shao, Yanbin 2 ; Sun, Yanchun 3 ;

作者机构： 1.Harbin Inst Technol, Sch Chem & Chem Engn, Dept Chem Mat, 92 West Dazhi St, Harbin 150001, Heilongjiang, Peoples R China

2.Harbin Inst Technol, Acad Fundamental & Interdisciplinary Sci, 92 West Dazhi St, Harbin 150001, Heilongjiang, Peoples R China

3.Chinese Acad Fishery Sci, Heilongjiang River Fishery Res Inst, Harbin 150001, Heilongjiang, Peoples R China

关键词： Carbon Nanodots;Photoluminescence Property;Doping;Fe3+ Sensing

期刊名称：JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY （ 影响因子：1.134； 五年影响因子：0.999 ）

ISSN： 1533-4880

年卷期： 2018 年 18 卷 6 期

页码：

收录情况： SCI

摘要： Nitrogen and silicon co-doped carbon nanodots (N/Si-CDs) were synthesized by one-step hydrothermal carbonization of folic acid and 3-aminopropyl trimethoxy silane with the assistance of glycerol. The resultant N/Si-CDs present intense excitation-independent photoluminescence (PL) emission owing to their monodisperse sizes and specific surface states. In comparison to nitrogen single doped CDs (N-CDs), the co-doped N/Si-CDs possess better PL properties following different emission manner due to the synergistic effects of the nitrogen and silicon dopants. Besides, the functionalized surfaces of N/Si-CDs endow them with superior solubility and stability. The as-synthesized N/Si-CDs demonstrate selective and sensitive fluorescence response to Fe3+, which could be explained by the PL quenching effects of Fe3+ on N/Si-CDs. Based on this finding, the quantitative analysis of aqueous Fe3+ by N/Si-CDs was established, showing good linearity in a range of 10 nM similar to 45 mu M and good sensitivity with a detection limit of 3.8 nM, so did for the detection of Fe3+ in fetal bovine serum (FBS) spiked samples. Therefore, the N/Si-CDs as a novel fluorescence probe hold promising for monitoring environmental and clinical Fe3+.

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