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Perovskite LaMnO3 Composite Graphene Carbon Nitride g-C3N4 Improves the Photocatalytic Performance of Tetracycline Degradation

文献类型： 外文期刊

作者： Lu, Ming 1 ; Dong, Jiaqi 1 ; Hu, Mingzhu 1 ; Cheng, Guofeng 2 ; Lv, Juan 1 ;

作者机构： 1.Univ Shanghai Sci & Technol, Sch Environm & Architecture, Shanghai 200093, Peoples R China

2.Chinese Acad Fishery Sci, Fishery Machinery & Instrument Res Inst, Shanghai 200092, Peoples R China

关键词： photocatalysis; LaMnO3/g-C3N4; visible light; z-scheme mechanism

期刊名称：WATER （ 影响因子：3.4； 五年影响因子：3.5 ）

ISSN：

年卷期： 2023 年 15 卷 8 期

页码：

收录情况： SCI

摘要： With the extensive use and improper treatment of antibiotics, antibiotic pollution in aquaculture wastewater has become increasingly severe. Tetracycline antibiotics have become one of the most commonly used fishery antibiotics. In this study, a Z-scheme heterostructure LaMnO3/g-C3N4 was constructed by the sol-gel method as a photocatalyst to degrade tetracycline, and the influence of anions on the degradation effect was investigated. The LaMnO3/g-C3N4 hybrid was successfully constructed by scanning electron microscope, Fourier transform infrared spectrum, and X-ray diffraction. The results of degradation experiments demonstrated that the maximum tetracycline degradation efficiency of LaMnO3/g-C3N4-10 (LMO/CN-10) was 80%, the removal rate of TC decreased from 71% to 48% when the concentration of chloride ions increased from 0 mM to 10 mM, and the removal rate of TC decreased from 75% to 28% when the concentration of carbonate ions increased from 0 mM to 10 mM. This enhanced photocatalytic activity was attributed to the formation of a Z-scheme structure that promoted the separation of photoinduced electron holes while maintaining its own strong redox ability. Finally, the photocatalytic mechanism was designed based on the free radical trapping experiment, electrochemical impedance, and photoluminescence spectra, providing an opportunity for the construction of a new photocatalyst for the treatment of aquaculture tailwater in the future.

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