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Removal of Phosphate from Aqueous Solution by Zeolite-Biochar Composite: Adsorption Performance and Regulation Mechanism

文献类型： 外文期刊

作者： Deng, Zhaoxia 1 ; Gu, Shangyi 1 ; Cheng, Hongguang 2 ; Xing, Dan 3 ; Twagirayezu, Gratien 4 ; Wang, Xi 2 ; Ning, Wenjing 2 ; Mao, Mingming 1 ;

作者机构： 1.Guizhou Univ, Coll Resources & Environm Engn, Guiyang 550025, Peoples R China

2.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Peoples R China

3.Guizhou Acad Agr Sci, Inst Pepper Guiyang, Guiyang 550000, Peoples R China

4.Lanzhou Jiaotong Univ, Sch Environm & Municipal Engn, Lanzhou 730070, Peoples R China

5.Huazhong Agr Univ, Coll Resource & Environm, Key Lab Arable Land Conservat Middle & Lower Reac, Minist Agr, Wuhan 430070, Peoples R China

6.Yangtze Univ, Coll Resources & Environm, Wuhan 430100, Peoples R China

关键词： phosphate; natural zeolite; biochar; composite; co-pyrolysis

期刊名称：APPLIED SCIENCES-BASEL （ 影响因子：2.838； 五年影响因子：2.921 ）

ISSN：

年卷期： 2022 年 12 卷 11 期

页码：

收录情况： SCI

摘要： Recently, rampant eutrophication induced by phosphorus enrichment in water has been attracting attention worldwide. However, the mechanisms by which phosphate can be eliminated from the aqueous environment remain unclear. This study was aimed at investigating the adsorption performance and regulation mechanisms of the zeolite-biochar composite for removing phosphate from an aqueous environment. To do this, physicochemical properties of the zeolite-biochar composite were assessed by Fourier transform infrared spectroscopy (FTIR), scanning electron microscopy (SEM), Brunauer-Emmett-Teller (BET) specific surface area (SSA) analyzer, and transmission electron microscopy (TEM). Adsorption tests were performed to evaluate the adsorption ability of the composite material for mitigating excess phosphorus in the aqueous environment. The findings evinced that the phosphorus removed by PZC 7:3 (pyrolyzed zeolite and corn straw at a mass ratio of 7:3) can reach 90% of that removed by biochar. The maximum adsorption capacities of zeolite, biochar, and PZC 7:3 were 0.69, 3.60, and 2.41 mg/g, respectively. The main mechanism of phosphate removal by PZC 7:3 was the formation of thin-film amorphous calcium-magnesium phosphate compounds through ligand exchange. This study suggests that PZC 7:3 is a viable adsorbent for the removal of phosphate from aquatic systems.

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